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Optical Multidimensional Coherent Spectroscopy

Optical Multidimensional Coherent Spectroscopy PDF Author: Associate Professor Hebin Li
Publisher: Oxford University Press
ISBN: 0192843869
Category : Science
Languages : en
Pages : 305

Book Description
This book provides an introduction to optical multidimensional coherent spectroscopy, a relatively new method of studying materials based on using ultrashort light pulses to perform spectroscopy. The technique has been developed and perfected over the last 25 years, resulting in multiple experimental approaches and applications to a broad array of systems ranging from atoms and molecules to solids and biological systems. Indeed, while this method is most often used by physical chemists, it is also relevant to materials of interest to physicists, which is the primary focus of this book. As well as an introduction to the method, the book also provides tutorials on the interpretation of the rather complex spectra that is broadly applicable across all subfields, and finishes with a survey of several emerging material systems and a discussion of future directions.

Optical Multidimensional Coherent Spectroscopy

Optical Multidimensional Coherent Spectroscopy PDF Author: Associate Professor Hebin Li
Publisher: Oxford University Press
ISBN: 0192843869
Category : Science
Languages : en
Pages : 305

Book Description
This book provides an introduction to optical multidimensional coherent spectroscopy, a relatively new method of studying materials based on using ultrashort light pulses to perform spectroscopy. The technique has been developed and perfected over the last 25 years, resulting in multiple experimental approaches and applications to a broad array of systems ranging from atoms and molecules to solids and biological systems. Indeed, while this method is most often used by physical chemists, it is also relevant to materials of interest to physicists, which is the primary focus of this book. As well as an introduction to the method, the book also provides tutorials on the interpretation of the rather complex spectra that is broadly applicable across all subfields, and finishes with a survey of several emerging material systems and a discussion of future directions.

Coherent Multidimensional Spectroscopy

Coherent Multidimensional Spectroscopy PDF Author: Minhaeng Cho
Publisher: Springer
ISBN: 9811397538
Category : Science
Languages : en
Pages : 404

Book Description
This book will fulfill the needs of time-domain spectroscopists who wish to deepen their understanding of both the theoretical and experimental features of this cutting-edge spectroscopy technique. Coherent Multidimensional Spectroscopy (CMDS) is a state-of-the-art technique with applications in a variety of subjects like chemistry, molecular physics, biochemistry, biophysics, and material science. Due to dramatic advancements of ultrafast laser technologies, diverse multidimensional spectroscopic methods utilizing combinations of THz, IR, visible, UV, and X-ray radiation sources have been developed and used to study real time dynamics of small molecules in solutions, proteins and nucleic acids in condensed phases and membranes, single and multiple excitons in functional materials like semiconductors, quantum dots, and solar cells, photo-excited states in light-harvesting complexes, ions in battery electrolytes, electronic and conformational changes in charge or proton transfer systems, and excess electrons and protons in water and biological systems.

Two-Dimensional Optical Spectroscopy

Two-Dimensional Optical Spectroscopy PDF Author: Minhaeng Cho
Publisher: CRC Press
ISBN: 1420084305
Category : Medical
Languages : en
Pages : 396

Book Description
Two-Dimensional Optical Spectroscopy discusses the principles and applications of newly emerging two-dimensional vibrational and optical spectroscopy techniques. It provides a detailed account of basic theory required for an understanding of two-dimensional vibrational and electronic spectroscopy. It also bridges the gap between the formal developm

Atomic and Laser Spectroscopy

Atomic and Laser Spectroscopy PDF Author: Alan Corney
Publisher: OUP Oxford
ISBN: 0191526339
Category : Science
Languages : en
Pages : 782

Book Description
This book discusses many advances in optical physic, and is aimed at advanced undergraduates taking courses in atomic physics, or graduate students in the fields of lasers, astrophysics, and physical chemistry. The book is intended mainly for experimentalists, and the interaction of electromagnetic radiation with free atoms is introduced using classical or semi-classical calculations wherever possible. Topics discussed include the spontaneous emission of radiation, stimulated transitions and the properties of gas and turnable dye lasers, and the physics and applications of resonance fluorescence, optical double resonance, optical pumping, and atomic beam magnetic resonance experiments.

Principles of Nonlinear Optical Spectroscopy

Principles of Nonlinear Optical Spectroscopy PDF Author: Shaul Mukamel
Publisher: Oxford University Press on Demand
ISBN: 9780195132915
Category : Science
Languages : en
Pages : 543

Book Description
This textbook presents a systematic and unifying viewpoint for a wide class of nonlinear spectroscopic techniques in time domain and frequency domain. It is directed towards active researchers in physics, optics, chemistry, and materials science, as well as graduate students who enter this complex and rapidly developing field. Nonlinear optical interactions of laser fields with matter provide powerful spectroscopic tools for the understanding of microscopic interactions and dynamic processes. One of the major obstacles facing researchers in this field, however, is the flood of experimental techniques and terminologies, which create a serious language barrier. The general microscopic correlation function approach to the nonlinear optical response developed in this book is essential for understanding the relationships among different techniques and a comparison of their information content, the design of new measurements, and for a systematic comparison of the optical response of different systems such as dyes in solutions, atoms and molecules in the gas phase, liquids, molecular aggregates and superlatives, and semiconductor nanostructures. The approach is based on formulating the nonlinear response by representing the state of matter by the density matrix and following its evolution on Liouville space. Current active research areas such as femtosecond time-domain techniques, semi-classical and wave-packet dynamics, pulse shaping, pulse locking, exciton confinement, and the interplay of electronic, nuclear and field coherence are emphasized. The material has been developed from the author's highly successful interdisciplinary course at the University of Rochester attended by science and engineering graduate students.

Concepts and Methods of 2D Infrared Spectroscopy

Concepts and Methods of 2D Infrared Spectroscopy PDF Author: Peter Hamm
Publisher: Cambridge University Press
ISBN: 1139497073
Category : Science
Languages : en
Pages : 297

Book Description
2D infrared (IR) spectroscopy is a cutting-edge technique, with applications in subjects as diverse as the energy sciences, biophysics and physical chemistry. This book introduces the essential concepts of 2D IR spectroscopy step-by-step to build an intuitive and in-depth understanding of the method. This unique book introduces the mathematical formalism in a simple manner, examines the design considerations for implementing the methods in the laboratory, and contains working computer code to simulate 2D IR spectra and exercises to illustrate involved concepts. Readers will learn how to accurately interpret 2D IR spectra, design their own spectrometer and invent their own pulse sequences. It is an excellent starting point for graduate students and researchers new to this exciting field. Computer codes and answers to the exercises can be downloaded from the authors' website, available at www.cambridge.org/9781107000056.

Two-Dimensional Correlation Spectroscopy

Two-Dimensional Correlation Spectroscopy PDF Author: Isao Noda
Publisher: John Wiley & Sons
ISBN: 0470012390
Category : Science
Languages : en
Pages : 310

Book Description
A valuable tool for individuals using correlation spectroscopy and those that want to start using this technique. Noda is known as the founder of this technique, and together with Ozaki, they are the two biggest names in the area First book on 2D vibrational and optical spectroscopy - single source of information, pulling together literature papers and reveiws Growing number of applications of this methodology - book now needed for people thinking of using this technique Limitations and benefits discussed and comparisons made with 2D NMR Discusses 20 optical and vibrational spectroscopy (IR, Raman, UV, Visible)

Semiconductor Nanostructures

Semiconductor Nanostructures PDF Author: Dieter Bimberg
Publisher: Springer Science & Business Media
ISBN: 3540778993
Category : Technology & Engineering
Languages : en
Pages : 369

Book Description
Reducing the size of a coherently grown semiconductor cluster in all three directions of space to a value below the de Broglie wavelength of a charge carrier leads to complete quantization of the energy levels, density of states, etc. Such “quantum dots” are more similar to giant atoms in a dielectric cage than to classical solids or semiconductors showing a dispersion of energy as a function of wavevector. Their electronic and optical properties depend strongly on their size and shape, i.e. on their geometry. By designing the geometry by controlling the growth of QDs, absolutely novel possibilities for material design leading to novel devices are opened. This multiauthor book written by world-wide recognized leaders of their particular fields and edited by the recipient of the Max-Born Award and Medal 2006 Professor Dieter Bimberg reports on the state of the art of the growing of quantum dots, the theory of self-organised growth, the theory of electronic and excitonic states, optical properties and transport in a variety of materials. It covers the subject from the early work beginning of the 1990s up to 2006. The topics addressed in the book are the focus of research in all leading semiconductor and optoelectronic device laboratories of the world.

Optical Properties And Spectroscopy Of Nanomaterials

Optical Properties And Spectroscopy Of Nanomaterials PDF Author: Jin Zhong Zhang
Publisher: World Scientific
ISBN: 981446936X
Category : Technology & Engineering
Languages : en
Pages : 400

Book Description
Optical properties are among the most fascinating and useful properties of nanomaterials and have been extensively studied using a variety of optical spectroscopic techniques. A basic understanding of the optical properties and related spectroscopic techniques is essential for anyone who is interested in learning about nanomaterials of semiconductors, insulators or metal. This is partly because optical properties are intimately related to other properties and functionalities (e.g. electronic, magnetic, and thermal) that are of fundamental importance to many technological applications, such as energy conversion, chemical analysis, biomedicine, optoelectronics, communication, and radiation detection.Intentionally designed for upper-level undergraduate students and beginning graduate students with some basic knowledge of quantum mechanics, this book provides the first systematic coverage of optical properties and spectroscopic techniques of nanomaterials.

Development of Coherent Two-dimensional Spectroscopy at Optical Frequencies and Application to Model Chromophores

Development of Coherent Two-dimensional Spectroscopy at Optical Frequencies and Application to Model Chromophores PDF Author: Hélène Seiler
Publisher:
ISBN:
Category :
Languages : en
Pages :

Book Description
"Ultrafast coherent multi-dimensional spectroscopies are a powerful set of techniques used to unravel complex processes. These processes range from electronic coherences in molecular chromophores to many-body interactions in quantum-confined materials. Yet these spectroscopies remain challenging to implement at the high frequencies of vibrational and electronic transitions, thereby limiting their widespread use. The work herein demonstrates three significant methodological improvements of two-dimensional spectroscopy at optical frequencies, followed by applications of the method on two different systems. First, we introduce a hollow-fibre setup for the production of broadband visible pulses. This source is comparatively simple to operate, and yields stable, 45 [mu]J pulses over the 520-700 nm region. Second, we demonstrate the feasibility of two-dimensional electronic spectroscopy in a single beam. By appropriately modulating the phases of the pulses within the beam,we show that it is possible to directly read out the relevant optical signals. This work shows that one needs neither complex beam geometries nor complex detection schemes in order to measure 2D spectra at optical frequencies. Finally, we introducea setup for complete and independent polarization control of each pulse in the sequence. Together, these methodological improvements represent important enabling steps towards the longstanding goal of achieving an "Optical NMR", and extendsthe realm of all-optical multi-dimensional spectroscopies to spatially heterogeneous samples. The methods are applied on two classes of systems. The model system Nile Blue is used to validate the performance of the instrument. The spectrometeris then used to reveal new processes in colloidal semiconductor CdSe nanocrystals, a system of contemporary interest." --