Irradiation Behavior of Uranium-fissium Alloys. EBR-II Project PDF Download
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Author: J. H. Kittel Publisher: ISBN: Category : Irradiation Languages : en Pages : 46
Book Description
A series of uranium-fissium and uranium-fissium-zirconium alloys was irradiated in thermal test reactors to study the relationship of dimensional stability to alloy composition, thermal cycling, burnup, irradiation temperature, post-irradiation heating, and cladding restraint. None of the alloy compositions tested showed irradiation behavior superior to the uranium-5 wt./% fissium alloy that has been used as driver fuel in EBR-II since it began operation. This alloy is among those uranium-base alloys most capable of resisting high-temperature irradiation swelling. None of the alloys showed evidence of the reversion to the metastable gamma phase that has been observed in comparable uranium-molybdenum alloys. Swelling of uranium-fissium alloys was effectively restrained by most of the 0.009-inch thick cladding materials investigated. Local hydrostatic forces due to swelling of the fuel caused the fuel to extrude extensively out of small vent holes in the cladding. Little axial fuel movement occurred within the cladding, however, even when the upper fuel surface was entirely unrestrained.
Author: J. H. Kittel Publisher: ISBN: Category : Irradiation Languages : en Pages : 46
Book Description
A series of uranium-fissium and uranium-fissium-zirconium alloys was irradiated in thermal test reactors to study the relationship of dimensional stability to alloy composition, thermal cycling, burnup, irradiation temperature, post-irradiation heating, and cladding restraint. None of the alloy compositions tested showed irradiation behavior superior to the uranium-5 wt./% fissium alloy that has been used as driver fuel in EBR-II since it began operation. This alloy is among those uranium-base alloys most capable of resisting high-temperature irradiation swelling. None of the alloys showed evidence of the reversion to the metastable gamma phase that has been observed in comparable uranium-molybdenum alloys. Swelling of uranium-fissium alloys was effectively restrained by most of the 0.009-inch thick cladding materials investigated. Local hydrostatic forces due to swelling of the fuel caused the fuel to extrude extensively out of small vent holes in the cladding. Little axial fuel movement occurred within the cladding, however, even when the upper fuel surface was entirely unrestrained.
Author: J. H. Kittel Publisher: ISBN: Category : Irradiation Languages : en Pages : 0
Book Description
A series of uranium-fissium and uranium-fissium-zirconium alloys was irradiated in thermal test reactors to study the relationship of dimensional stability to alloy composition, thermal cycling, burnup, irradiation temperature, post-irradiation heating, and cladding restraint. None of the alloy compositions tested showed irradiation behavior superior to the uranium-5 wt./% fissium alloy that has been used as driver fuel in EBR-II since it began operation. This alloy is among those uranium-base alloys most capable of resisting high-temperature irradiation swelling. None of the alloys showed evidence of the reversion to the metastable gamma phase that has been observed in comparable uranium-molybdenum alloys. Swelling of uranium-fissium alloys was effectively restrained by most of the 0.009-inch thick cladding materials investigated. Local hydrostatic forces due to swelling of the fuel caused the fuel to extrude extensively out of small vent holes in the cladding. Little axial fuel movement occurred within the cladding, however, even when the upper fuel surface was entirely unrestrained.
Author: J. A. Horak Publisher: ISBN: Category : Alloys Languages : en Pages : 40
Book Description
A total of 35 specimens of U-Pu-fissium alloy and 2 specimens of U-10 wt% Pu-5 wt% Mo alloy were irradiated as a part of the fuel-alloy development program for fast breeder reactors at Argonne National Laboratory. Total atom burnups ranged from 1.0 to 1.8% at maximum fuel temperatures ranging from 230 to 470 deg C. Emphasis was placed on the EBR-II Core-III reference fuel material, which is an injection-cast, U-20 wt% Pu-10 wt% fissium alloy. It was found that this material begins to swell catastrophically at irradiation temperatures above 370 deg C. The ability of the fuel to resist swelling did not appear to vary appreciably with minor changes in zirconium or fissium content. Decreasing the Pu to 10 wt%, however, significantly improved the swelling behavior of the alloy. Both pour-cast and thermally cycled material and pour-cast, extruded, and thermally cycled material appeared to be more stable under irradiation than injection-cast material. Under comparable irradiation conditions, the specimens of U-20 wt% Pu- 5 wt% Mo alloy were less dimensionally stable than the U-Pu-fissium alloys investigated.
Author: J. A. Horak Publisher: ISBN: Category : Irradiation Languages : en Pages : 46
Book Description
Twelve 0.22-in.-diameter fuel specimens containing a longitudinal central vent and clad with 0.010 in. of Type 304 stainless steel were irradiated to evaluate the effect of restraint and a central vent on fuel element stability. The cladding of 10 of the specimens contained porous end plugs to vent any released fission gas and thus to minimize the buildup of gas pressure within the stainless steel cladding. The specimens consisted of a 20% enriched uranium--2 wt% zirconium alloy core surrounded by a natural uranium--2 wt% zirconium alloy sleeve. Eight of the specimens were irradiated to burnups of the enriched core of 6.9 to 12.8% of all atoms (1.2 to 2.2 at.% of the duplex assembly) at maximum fuel temperatures ranging from 280 to 760 deg C. Most of the clad specimens exhibited negligible volume increases as a result of irradiation. Two specimens containing central vents but unclad were irradiated together with the clad specimens in an attempt to differentiate between the effects due to a central vent and the effects due to cladding. The central vent in itself did not appear to reduce the swelling characteristics of the alloy. Mechanical restraint appeared to have extended the useful operating temperatures of the metallic fuel alloy by at least 200 deg C and also greatly extended the burnup levels to which the fuel could be irradiated.
Author: Publisher: ISBN: Category : Languages : en Pages :
Book Description
A total of 35 specimens of U-Pu-fissium alloy and 2 specimens of U-10 wt% Pu-5 wt% Mo alloy were irradiated as a part of the fue1-alloy development program for fast breeder reactors at Argonne National Laboratory. Total atom burnups ranged from 1.0 to 1.8% at maximum fuel temperatures ranging from 230 to 470 deg C. Emphasis was placed on the EBR-II Core-III reference fuel material, which is an injection-cast, U-20 wt% Pu-10 wt% fissium alloy. lt was found that this material begins to swell catastrophically at irradiation temperatures above 370 deg C. The ability of the fuel to resist swelling did not appear to vary appreciably with minor changes in Zr or fissium content. Decreasing the Pu to 10 wt%, however, significantly improved the swelling behavior of the alloy. Both pourcast and thermally cycled material and pour-cast, extruded, and thermally cycled material appeared to be more stable under irradiation than injection-cast material. Under comparable irradiation conditions, the specimens of U-20 wt% Pu- 5 wt% Mo alloy were less dimensionally stable than the U-Pu-fissium alloys investigated. (auth).
Author: J. H. Kittel Publisher: ISBN: Category : Irradiation Languages : en Pages : 40
Book Description
The fuel material specified for the Mark III core of EBR-I was uranium-2 wt. % zirconium alloy coextruded with Zircaloy-2 cladding. From previous work on swaged or rolled uranium-2 wt% zirconium alloy, it was anticipated that the extruded alloy would be dimensionally unstable under irradiation unless stabilized by suitable heat treatment. In order to determine an effective heat treatment, irradiation studies were made on both clad and unclad extruded uranium-2 wt.% zirconium alloy specimens at irradiation temperature estimated at 200 to 750 deg C. The irradiation specimens included material with three different heat treatments, selected on the basis of previous studies, and material transient melted in its cladding. For unclad specimens, it was found that the irradiation temperature strongly influenced the various irradiation growth rates resulting from different heat treatments. Growth rates of the clad specimens were relatively insensitive to either irradiation temperature or prior heat treatment. An exception was the transient-melted material, which shortened under irradiation. The cladding had only limited ability to restrain the swelling rates of specimens irradiated at the more elevated temperatures. Clad transient-melted material was found to be most resistant to high-temperature swelling under irradiation. The results of the present study combined with observations in earlier investigations resulted in a recommendation that the reference heat treatment for the core consist of gamma solution at 800 deg C followed by isothermal transformation at 690 deg C.
Author: Publisher: ISBN: Category : Languages : en Pages :
Book Description
Twelve 0.22-in.-diameter fuel specimens containing a longitudinal central vent and clad with 0.010 in. of Type 304 stainless steel were irradiated to evaluate the effect of restraint and a central vent on fuel element stability. The cladding of 10 of the specimens contained porous end plugs to vent any released fission gas and thus to minimize the buildup of gas pressure within the stainless steel cladding. The specimens consisted of a 20% enriched uranium--2 wt% zirconium alloy core surrounded by a natural uranium--2 wt% zirconium alloy sleeve. Eight of the specimens were irradiated to burnups of the enriched core of 6.9 to 12.8% of all atoms (1.2 to 2.2 at.% of the duplex assembly) at maximum fuel temperatures ranging from 280 to 760 deg C. Most of the clad specimens exhibited negligible volume increases as a result of irradiation. Two specimens containing central vents but unclad were irradiated together with the clad specimens in an attempt to differentiate between the effects due to a central vent and the effects due to cladding. The central vent in itself did not appear to reduce the swelling characteristics of the alloy. Mechanical restraint appeared to have extended the useful operating temperatures of the metallic fuel alloy by at least 200 deg C and also greatly extended the burnup levels to which the fuel could be irradiated. (auth).
Author: J. H. Kittel
Author: J. H. Kittel
Author: J. H. Kittel
Author: J. A. Horak
Author: J. A. Horak
Author: 
Author: Gordon G. Bentle
Author: D. I. Sinizer
Author: J. H. Kittel
Author: R. D. Leggett
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