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Characterization and Source Apportionment of Ambient PM2.5 in Atlanta, Georgia

Characterization and Source Apportionment of Ambient PM2.5 in Atlanta, Georgia PDF Author: Bo Yan
Publisher:
ISBN:
Category : Air
Languages : en
Pages :

Book Description
Various airborne PM2.5 samples were collected in the metropolitan Atlanta and surrounding areas, which are directly impacted or dominated by on-road mobile and other typical urban emissions, regional transport sources, prescribed burning plumes, wildfire plumes, as well as secondary sources with anthropogenic and biogenic nature in origin. Detailed PM2.5 chemical speciation was conducted including over one hundred of GC/MS-quantified organic compounds, organic carbon (OC), water-soluble organic carbon (WSOC), elemental carbon (EC), ionic species, and tens of trace metals. Day-night, seasonal and spatial variations of PM2.5 characterization were also studied. Contributions of PM2.5 major sources were identified quantitatively through the receptor source apportionment models. These modeling results, especially on-road mobile source contributions and secondary organic carbon (SOC) were assessed by multiple approaches. Furthermore, new season- and location-specific source profiles were developed in this research to reflect real-world and representative local emission characterizations of on-road mobile sources, aged prescribed burning plumes, and wildfire plumes. Secondary organic aerosol (SOA), a major component of PM2.5 in the summer, was also explored for sources and contributions.

Characterization and Source Apportionment of Ambient PM2.5 in Atlanta, Georgia

Characterization and Source Apportionment of Ambient PM2.5 in Atlanta, Georgia PDF Author: Bo Yan
Publisher:
ISBN:
Category : Air
Languages : en
Pages :

Book Description
Various airborne PM2.5 samples were collected in the metropolitan Atlanta and surrounding areas, which are directly impacted or dominated by on-road mobile and other typical urban emissions, regional transport sources, prescribed burning plumes, wildfire plumes, as well as secondary sources with anthropogenic and biogenic nature in origin. Detailed PM2.5 chemical speciation was conducted including over one hundred of GC/MS-quantified organic compounds, organic carbon (OC), water-soluble organic carbon (WSOC), elemental carbon (EC), ionic species, and tens of trace metals. Day-night, seasonal and spatial variations of PM2.5 characterization were also studied. Contributions of PM2.5 major sources were identified quantitatively through the receptor source apportionment models. These modeling results, especially on-road mobile source contributions and secondary organic carbon (SOC) were assessed by multiple approaches. Furthermore, new season- and location-specific source profiles were developed in this research to reflect real-world and representative local emission characterizations of on-road mobile sources, aged prescribed burning plumes, and wildfire plumes. Secondary organic aerosol (SOA), a major component of PM2.5 in the summer, was also explored for sources and contributions.

Characterization and Source Apportionment of PM2.5 in the Southeastern United States

Characterization and Source Apportionment of PM2.5 in the Southeastern United States PDF Author: Sangil Lee
Publisher:
ISBN:
Category :
Languages : en
Pages : 126

Book Description
Uncertainties of source apportionment results are important for not only health studies but also policy analysis and decision making as they can affect confidence in the final results. They should be investigated for an appropriate application of source apportionment results. Thus, uncertainty and its contributors were estimated by propagating uncertainties in input data using Monte Carlo analysis.

Sources and Composition of Ambient Particulate Matter

Sources and Composition of Ambient Particulate Matter PDF Author: Manousos-Ioannis Manousakas
Publisher: MDPI
ISBN: 303650995X
Category : Science
Languages : en
Pages : 246

Book Description
Research related to ambient particulate matter (PM) remains very relevant today due to the adverse effects that PM have on human health. PM are pollutants with varying chemical compositions and may originate from multiple emission sources, which directly affects their toxicity. To formulate effective control and mitigation strategies, it is necessary to identify PM sources and to estimate their influence on ambient PM concentration, a process that is known as source apportionment (SA). Depending on the geographical location and characteristics of an area, many anthropogenic and natural sources may contribute to PM concentration levels, such as dust resuspension, sea salt, traffic, secondary aerosol formation, industrial emissions, ship emissions, biomass burning, power plant emissions, etc. Different methodological approaches have been used over the years to study the aforementioned topics, but some scientific challenges remain, mainly related to the following subjects: real-time chemical analysis and SA, uncertainty estimation of SA results, and analytical optimization for PM samples. Additionally, there are areas in the world for which the results regarding composition and sources of PM are still scarce. The objective of this collection was to include studies on all aspects of PM chemical characterization and source apportionment regarding the inorganic and/or organic fractions of PM.

Particulate Modeling and Control Strategy for Atlanta, Georgia

Particulate Modeling and Control Strategy for Atlanta, Georgia PDF Author: Sun-kyoung Park
Publisher:
ISBN:
Category : Air
Languages : en
Pages :

Book Description
Particles reduce visibility, change climate, and affect human health. In 1997, the National Ambient Air Quality Standard (NAAQS) for PM2.5 (particles less than 2.5 mm) was promulgated. The annual mean PM2.5 mass concentrations in Atlanta, Georgia exceed the standard, and control is needed. The first goal of this study is to develop the control strategies of PM2.5 in Atlanta, Georgia. Based on the statistical analysis of measured data, from 22% to 40% of emission reductions are required to meet the NAAQS at 95% CI. The estimated control levels can be tested using the Community Multiscale Air Quality (CMAQ) model to better assess if the proposed levels will achieve sufficient reduction in PM2.5. The second goal of this study is to analyze various uncertainties residing in CMAQ. For the model to be used in such applications with confidence, it needs to be evaluated. The model performance is calculated by the relative agreement between volume-averaged predictions and point measurements. Up to 14% of the model error for PM2.5 mass is due to the different spatial scales of the two values. CMAQ predicts PM2.5 mass concentrations reasonably well, but CMAQ significantly underestimates PM2.5 number concentrations. Causes of the underestimation include that assumed inaccurate particle density and particle size of the primary emissions in CMAQ, in addition to the expression of the particle size with three lognormal distributions. Also, the strength and limitations of CMAQ in performing PM2.5 source apportionment are compared with those of the Chemical Mass Balance with Molecular Markers. Finally, the accuracy of emissions, one of the important inputs of CMAQ, is evaluated by the inverse modeling. Results show that base level emissions for CO and SO2 sources are relatively accurate, whereas NH3, NOx, PEC and PMFINE emissions are overestimated. The emission adjustment for POA and VOC emissions is significantly different among regions.

Air-quality Modeling and Source-apportionment of Fine Particulate Matter: Implications and Applications in Time-series Health Studies

Air-quality Modeling and Source-apportionment of Fine Particulate Matter: Implications and Applications in Time-series Health Studies PDF Author: Amit Marmur
Publisher:
ISBN: 9781109871142
Category :
Languages : en
Pages : 186

Book Description
Air-quality modeling tools may be useful in such investigations of the health effects of air-pollution and PM2.5 specifically. Emissions-based three-dimensional air quality models may introduce several benefits when applied in epidemiologic studies, such as improved spatial representativeness and availability/continuity of data, as well as information on source impacts. Receptor-based models are a common tool for apportioning of ambient levels of pollutants among the major contributing sources, and can be useful in discerning the relative health impacts of different sources.

Environmental Health Perspectives

Environmental Health Perspectives PDF Author:
Publisher:
ISBN:
Category : Environmental health
Languages : en
Pages : 1576

Book Description


Air Pollution And Health

Air Pollution And Health PDF Author: Jon G Ayres
Publisher: World Scientific
ISBN: 1783261919
Category : Medical
Languages : en
Pages : 266

Book Description
This invaluable volume, the third in the series Air Pollution Reviews, addresses particular questions relating to air pollution and its effect on health. It deals with the impact of nasal disease on lung exposure, how pollutants are distributed within the lung, and the uncertainties with regard to defining the dose to the lung. It takes a tangential look at the lung dose by exploring the possibility of obtaining clues from occupational medicine.Toxicologically, the book examines the possible methodology for exploring how particles and their toxicity can be investigated, and looks into the cardio-toxic effects of air pollution. The effects of pollutant mixtures are compared with those of individual pollutants. In addition, the question of the importance of acid aerosols is tackled.Epidemiologically, the book deals with the problems associated with point sources as opposed to diffuse sources of air pollution, and considers whether the health effects of air pollution can be adequately quantified.These areas, though difficult, need to be addressed, in order to develop our knowledge of the health effects of air pollution. In this volume, a strong panel of authors treat the issues. They have raised questions but at the same time succeeded in solving a number of problems.

Source Apportionment of PM2.5 in Milan by PMF Receptor Model

Source Apportionment of PM2.5 in Milan by PMF Receptor Model PDF Author: Sanja Savic
Publisher: LAP Lambert Academic Publishing
ISBN: 9783330345737
Category :
Languages : en
Pages : 80

Book Description
This case study discusses the application of a multivariate receptor model, the EPA PMF 5.0 to the PM2.5 dataset from Lombardy region in Italy. The aim of the study is to perform source apportionment investigation of the applied dataset and identify different PM2.5 sources that greatly impact the composition of particulate matter in the studied region. PMF model evaluates contribution to diverse source types of measured PM2.5 concentrations by investigating chemical composition of ambient pollution samples. As a type of receptor models, PMF used as an input data, PM concentrations and their relative chemical specification and provides as an outcome the number of sources, their composition and the source contributions. The analysis of total annual PM2.5 mass concentration revealed presence of 6 sources (secondary sulfate, traffic non-exhaust, biomass combustion/break wear, domestic heating, re-suspended soil dust and secondary nitrate).

Synergic Influence of Gaseous, Particulate, and Biological Pollutants on Human Health

Synergic Influence of Gaseous, Particulate, and Biological Pollutants on Human Health PDF Author: Jozef S. Pastuszka
Publisher: CRC Press
ISBN: 1498715125
Category : Medical
Languages : en
Pages : 314

Book Description
Synergic Influence of Gaseous, Particulate, and Biological Pollutants on Human Health is a unique merger of two divergent parts. The first part is a presentation of the existing knowledge on the characteristics of basic air pollutants and their documented impact on human health. The focus is on the main gaseous, airborne particles (including fiber

Integrated Air Quality Management

Integrated Air Quality Management PDF Author: Nguyen Thi Kim Oanh
Publisher: CRC Press
ISBN: 1439862257
Category : Law
Languages : en
Pages : 443

Book Description
The steady growth in the number of vehicles on the road, heavy reliance on coal, use of dirty fuels for residential combustion, and extensive open burning are some of the major factors leading to the progressive deterioration of air quality in developing countries in Asia. And despite efforts to establish and implement air quality measurement systems, the development of infrastructure, environmental technology, and management practices continues to lag behind the rate of emission increase. Based on ten years of coordinated research, Integrated Air Quality Management: Asian Case Studies discusses technical and policy tools for the integrated air quality management of developing countries in Asia. The book begins with an overview of major issues of air quality management practices in developing Asia and potential approaches to reduce pollution, including opportunities for integration of air quality improvement and climate migration strategies. It covers the methodology and results of fine particulate matter monitoring using traditional filter-based and satellite monitoring techniques. It examines the applications of a 3D dispersion modeling tool for urban and regional air quality management focusing on surface ozone, fine particulate matter, and acid deposition. The final chapters discuss innovative control technologies for gaseous air pollutants and illustrate the integrated air quality management in developing Asia through case studies for target source categories including agricultural residue field burning, vehicle emissions, brick kilns, and industrial VOC emission. Illustrated with case studies, this book presents an integrated air quality management methodology that employs technical and policy tools to achieve air quality goals. It includes technical information and policy recommendations based on the outcomes of several multi-year air quality research programs coordinated by the Asian Institute of Technology. The text combines fundamental information and advanced knowledge useful to large audiences dealing with subjects of integrated air quality management.