A proposal for the irradiation of uranium metal alloys PDF Download

Author: J. F. Walker
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Category :
Languages : en
Pages : 0

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Author: Gordon G. Bentle
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Category : Nuclear fuel elements
Languages : en
Pages : 76

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Author: T. I. Jones
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Category :
Languages : en
Pages : 0

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Author: M. P. Johnson
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Category : Molybdenum alloys
Languages : en
Pages : 38

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A series of experiments was designed to assess the suitability of uranium-molybdenum alloys as high-temperature, high-burnup fuels for advanced sodium cooled reactors. Specimens with molybdenum contents between 3 and 10% were subjected to capsule irradiation tests in the Materials Testing Reactor, to burnups up to 10,000 Mwd/MTU at temperatures between 800 and 1500 deg F. The results indicated that molybdenum has a considerable effect in reducing the swelling due to irradiation. For example. 3% molybdemum reduces the swelling from 25%, for pure uranium. to 7% at approximates 3,000 Mwd/MTU at 1270 deg F. Further swelling resistance can be gained by increasing the molybdenum content, but the amount gained becomes successively smaller. At higher irradiation levels, the amount of swelling rapidly becomes greater, and larger amounts of molybdenum are required to provide similar resistance. A limit of 7% swelling, at 900 deg F and an irradiation of 7,230 Mwd/ MTU, requires the use of 10% Nonemolybdenum in the alloy. The burnup rates were in the range of 2.0 to 4.0 x 10p13s fissiom/cc-sec. Small ternary additions of silicon and aluminum were shown to have a noticeable effect in reducing swelling when added to a U-3% Mo alloy base. Under the conditions of the present experiment, 0.26% silicon or 0.38% aluminum were equivalent to 1 to 1 1/2% molybdenum. The Advanced Sodium Cooled Reactor requires a fuel capable of being irradiated to 20,000 Mwd/MTU at temperatures up to 1500 deg C in metal fuel, or equivalent in ceramic fuel. It is concluded that even the highest molybdenum contents considered did not produce a fuel capable of operating satisfactorily under these conditions. The alloys would be useful, however, for less exacting conditions. The U-3% Mo alloy is capable of use up to 3,000 Mwd/MTU at temperatures of 1300 deg F before swelling becomes excessive. The addition of silicon and aluminum would increase this limit to at least 3,000 Mwd/MTU, and possibly more if the

Author: R. E. Hueschen
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Category : Irradiation
Languages : en
Pages : 60

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Category :
Languages : en
Pages : 0

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Category :
Languages : en
Pages : 5

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Postirradiation examinations were begun of a series of unrestrained dilute uranium alloy specimens irradiated to exposures up to 13,000 MWD/T in NaK-containing stainless steel capsules. This test, part of a program of development of uranium metal fuels for desalination and power reactors sponsored by the Division of Reactor Development and Technology, has the objective of defining the temperature and exposure limits of swelling resistance of the alloyed uranium. This paper discusses those test results.

Author: J. A. Horak
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Category : Alloys
Languages : en
Pages : 40

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A total of 35 specimens of U-Pu-fissium alloy and 2 specimens of U-10 wt% Pu-5 wt% Mo alloy were irradiated as a part of the fuel-alloy development program for fast breeder reactors at Argonne National Laboratory. Total atom burnups ranged from 1.0 to 1.8% at maximum fuel temperatures ranging from 230 to 470 deg C. Emphasis was placed on the EBR-II Core-III reference fuel material, which is an injection-cast, U-20 wt% Pu-10 wt% fissium alloy. It was found that this material begins to swell catastrophically at irradiation temperatures above 370 deg C. The ability of the fuel to resist swelling did not appear to vary appreciably with minor changes in zirconium or fissium content. Decreasing the Pu to 10 wt%, however, significantly improved the swelling behavior of the alloy. Both pour-cast and thermally cycled material and pour-cast, extruded, and thermally cycled material appeared to be more stable under irradiation than injection-cast material. Under comparable irradiation conditions, the specimens of U-20 wt% Pu- 5 wt% Mo alloy were less dimensionally stable than the U-Pu-fissium alloys investigated.

Author: J. H. Kittel
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Category : Irradiation
Languages : en
Pages : 46

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A series of uranium-fissium and uranium-fissium-zirconium alloys was irradiated in thermal test reactors to study the relationship of dimensional stability to alloy composition, thermal cycling, burnup, irradiation temperature, post-irradiation heating, and cladding restraint. None of the alloy compositions tested showed irradiation behavior superior to the uranium-5 wt./% fissium alloy that has been used as driver fuel in EBR-II since it began operation. This alloy is among those uranium-base alloys most capable of resisting high-temperature irradiation swelling. None of the alloys showed evidence of the reversion to the metastable gamma phase that has been observed in comparable uranium-molybdenum alloys. Swelling of uranium-fissium alloys was effectively restrained by most of the 0.009-inch thick cladding materials investigated. Local hydrostatic forces due to swelling of the fuel caused the fuel to extrude extensively out of small vent holes in the cladding. Little axial fuel movement occurred within the cladding, however, even when the upper fuel surface was entirely unrestrained.

Author: W. N. Hansen
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Category : Thorium alloys
Languages : en
Pages : 40

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