Synthesis and characterization of new transition metal complexes for catalytic oxidation and electrolytic proton reduction PDF Download

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Synthesis and characterization of new transition metal complexes for catalytic oxidation and electrolytic proton reduction

Synthesis and characterization of new transition metal complexes for catalytic oxidation and electrolytic proton reduction PDF Author: Olesea Cuzan
Publisher:
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Languages : en
Pages : 135

Book Description
Nowadays, the ability to synthesize new bioinspired metal catalysts to improve and broaden the spectrum of catalytic activity is of paramount importance for sustainable chemistry respectful for our environment. This thesis is focused on the design of transition metal complexes (copper and palladium) based on two different classes of organic ligands: benzotriazolyl-phenolates and phosphonates.Different original complexes based on palladium and copper were synthetized from benzotriazolyl-phenolate and phosphonates ligands. The characterization of the new compounds was performed by different physical and physico-chemical methods (electrochemistry, EPR, UV-vis, IR, X-ray crystallography) and quantum chemistry. The generation and characterization of different reduced and oxidized species helped us in the possible mechanisms determination. The obtained compounds were successfully employed as catalysts in different processes as: hydrogen production, alcohol oxidation and DNA cleavage.
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