Author: Shaul Mukamel
Publisher:
ISBN:
Category :
Languages : en
Pages : 15
Book Description
This research program resulted in 53 publications. 43 already appeared, 4 are accepted for publication, and 6 were submitted. These publications are listed at the end of the final report. The research focused in the following major areas: (1) molecular semi-classical dynamics in Liouville space; a unified description of vibrational relaxation nonlinear spectroscopy and rate processes; (ii) intramolecular vibrational redistribution; (iii) vibrational and radiative dynamics in molecular clusters; (iv) coherent and spontaneous Raman, fluorescence and four-wave mixing spectroscopy; (v) excitation transport, electron transfer, and localization in disordered molecular systems. The main accomplishments are summarized in the final report. Molecular semiclassical dynamics, Vibrational relaxation, Nonlinear spectroscopy, Energy transfer, Molecular systems. (MJM).
Intermolecular and Intramolecular Vibrational Relaxation and Energy Transfer
Author: Shaul Mukamel
Publisher:
ISBN:
Category :
Languages : en
Pages : 15
Book Description
This research program resulted in 53 publications. 43 already appeared, 4 are accepted for publication, and 6 were submitted. These publications are listed at the end of the final report. The research focused in the following major areas: (1) molecular semi-classical dynamics in Liouville space; a unified description of vibrational relaxation nonlinear spectroscopy and rate processes; (ii) intramolecular vibrational redistribution; (iii) vibrational and radiative dynamics in molecular clusters; (iv) coherent and spontaneous Raman, fluorescence and four-wave mixing spectroscopy; (v) excitation transport, electron transfer, and localization in disordered molecular systems. The main accomplishments are summarized in the final report. Molecular semiclassical dynamics, Vibrational relaxation, Nonlinear spectroscopy, Energy transfer, Molecular systems. (MJM).
Publisher:
ISBN:
Category :
Languages : en
Pages : 15
Book Description
This research program resulted in 53 publications. 43 already appeared, 4 are accepted for publication, and 6 were submitted. These publications are listed at the end of the final report. The research focused in the following major areas: (1) molecular semi-classical dynamics in Liouville space; a unified description of vibrational relaxation nonlinear spectroscopy and rate processes; (ii) intramolecular vibrational redistribution; (iii) vibrational and radiative dynamics in molecular clusters; (iv) coherent and spontaneous Raman, fluorescence and four-wave mixing spectroscopy; (v) excitation transport, electron transfer, and localization in disordered molecular systems. The main accomplishments are summarized in the final report. Molecular semiclassical dynamics, Vibrational relaxation, Nonlinear spectroscopy, Energy transfer, Molecular systems. (MJM).
Intermolecular and Intramolecular Vibrational Energy Transfer in Unimolecular Reaction Systems
Author: Yueh-neu Shih Lin
Publisher:
ISBN:
Category : Chemical reactions
Languages : en
Pages : 404
Book Description
Publisher:
ISBN:
Category : Chemical reactions
Languages : en
Pages : 404
Book Description
Intramolecular and Intermolecular Energy Transfer in Highly Vibrationally Excited Molecules
Author: F. Crim
Publisher:
ISBN:
Category :
Languages : en
Pages : 8
Book Description
The research described in this Final Report was directed at studying the dynamics of vibrationally excited molecules, which are important in many energetic environments. The first goal was assembly of an ultrafast laser system producing 1 mJ, 100 fs pulses of 800 nm light, and implementing nonlinear processes for converting those pulses to infrared and ultraviolet light. This system permitted the a direct measurement of the time for intramolecular vibrational energy flow in nitric acid (HONO2) initially prepared with two quanta of O-H bond stretching excitation. The measurements showed that energy flowed out of that initially excited vibration in 12 ps, a time consistent with a coupling matrix element of about 0.08 /cm. This result on an isolated molecule sets the stage for the a similar measurement in a liquid.
Publisher:
ISBN:
Category :
Languages : en
Pages : 8
Book Description
The research described in this Final Report was directed at studying the dynamics of vibrationally excited molecules, which are important in many energetic environments. The first goal was assembly of an ultrafast laser system producing 1 mJ, 100 fs pulses of 800 nm light, and implementing nonlinear processes for converting those pulses to infrared and ultraviolet light. This system permitted the a direct measurement of the time for intramolecular vibrational energy flow in nitric acid (HONO2) initially prepared with two quanta of O-H bond stretching excitation. The measurements showed that energy flowed out of that initially excited vibration in 12 ps, a time consistent with a coupling matrix element of about 0.08 /cm. This result on an isolated molecule sets the stage for the a similar measurement in a liquid.
Vibrational Relaxation and Photodissociation Dynamics in Solution
Author: Christopher George Elles
Publisher:
ISBN:
Category :
Languages : en
Pages : 256
Book Description
Publisher:
ISBN:
Category :
Languages : en
Pages : 256
Book Description
Vibrational and Rotational Relaxation in Gases
Author: James Dewe Lambert
Publisher: Oxford University Press, USA
ISBN:
Category : Language Arts & Disciplines
Languages : en
Pages : 168
Book Description
Publisher: Oxford University Press, USA
ISBN:
Category : Language Arts & Disciplines
Languages : en
Pages : 168
Book Description
Experimental Investigations of Intermolecular Vibrational Energy Transfer
Understanding Intramolecular and Intermolecular Contributions to Energy Relaxation
Author: Scott Nelson Goldie
Publisher:
ISBN:
Category : Energy transfer
Languages : en
Pages : 374
Book Description
Publisher:
ISBN:
Category : Energy transfer
Languages : en
Pages : 374
Book Description
Scientific and Technical Aerospace Reports
State-to-field Vibrational Energy Transfer in S1 Para-difluorobenzene
Molecular Dynamics and Spectroscopy by Stimulated Emission Pumping
Author: Hai-Lung Dai
Publisher: World Scientific
ISBN: 9789810221119
Category : Science
Languages : en
Pages : 1148
Book Description
Since the first stimulated emission pumping (SEP) experiments more than a decade ago, this technique has proven powerful for studying vibrationally excited molecules. SEP is now widely used by increasing numbers of research groups to investigate fundamental problems in spectroscopy, intramolecular dynamics, intermolecular interactions, and even reactions. SEP provides rotationally pre-selected spectra of vibrationally highly excited molecules undergoing large amplitude motions. A unique feature of SEP is the ability to access systematically a wide variety of extreme excitations localized in various parts of a molecule, and to prepare populations in specific, high vibrational levels. SEP has made it possible to ask and answer specific questions about intramolecular vibrational redistribution and the role of vibrational excitation in chemical reactions.
Publisher: World Scientific
ISBN: 9789810221119
Category : Science
Languages : en
Pages : 1148
Book Description
Since the first stimulated emission pumping (SEP) experiments more than a decade ago, this technique has proven powerful for studying vibrationally excited molecules. SEP is now widely used by increasing numbers of research groups to investigate fundamental problems in spectroscopy, intramolecular dynamics, intermolecular interactions, and even reactions. SEP provides rotationally pre-selected spectra of vibrationally highly excited molecules undergoing large amplitude motions. A unique feature of SEP is the ability to access systematically a wide variety of extreme excitations localized in various parts of a molecule, and to prepare populations in specific, high vibrational levels. SEP has made it possible to ask and answer specific questions about intramolecular vibrational redistribution and the role of vibrational excitation in chemical reactions.