Inelastic Neutron Scattering Studies of Novel Quantum Magnets PDF Download

Author: Kemp William Plumb
Publisher:
ISBN:
Category :
Languages : en
Pages :

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Author:
Publisher:
ISBN:
Category :
Languages : en
Pages : 203

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The behavior of magnetic systems in the extreme quantum limit is one of the most interesting forefront areas in condensed matter physics. This dissertation investigates two particularly interesting quantum magnets: LiVO2 and DMACuCl3. Systematic studies were performed on single crystal samples using different experimental techniques, especially inelastic neutron scattering. Detailed experimental results and corresponding model calculations are presented and discussed in this dissertation. LiVO2 is a good candidate to study the interplay between ʺmagnetic frustrationʺ and orbital ordering. V3+ ions in LiVO2 form a triangular lattice involving threefold degenerate t2g orbitals. LiVO2 undergoes a first order phase transition at Tt = 500 K accompanied by a large reduction of the magnetic susceptibility in the low temperature phase. The origin of this phase transition has been associated with a peculiar type of t2g orbital ordering resulting in the formation of vanadium trimer clusters with a spin-singlet ground state. Our inelastic neutron scattering experiments reveal multiple magnetic excitations with energy transfer as large as several hundreds of meV associated with the low temperature orbitally ordered phase. This can not be explained by a simple ʺspin-onlyʺ isolated trimer model. Model calculations including a Kugel-Khomskii orbital-ordering term yield qualitatively similar spectra suggesting that a new type of excitation, which we refer to as ʺcluster orbitonʺ, has been observed in LiVO2. DMACuCl3 was proposed as a S = 1/2 FM-AFM alternating-sign chain along the a-axis. However, our inelastic neutron scattering experiments indicate that the strong magnetic coupling in DMACuCl3 is along the b-axis, and the magnetic excitation spectrum is dominated by the FM-AFM alternating chain with J (subscript FM) = -1.2(1) meV and J(subscript AFM) = 1.3(2) meV. Furthermore, recent studies show that DMACuCl3 undergoes a structural phase transition at Tt = 285 K. Below T(subscript t), the low temperature crystal structure suggests that DMACuCl3 contains two types of dimers: FM and AFM dimers. Inelastic neutron scattering results suggest a two chain model along the b-axis for DMACuCl3. This research is conducted under the supervision of the authorʹs advisors: Dr. David G. Mandrus at material science and technology division and Dr. Stephen E. Nagler at center for neutron scattering, Oak Ridge National Laboratory.

Author: Chiron Jeeb Mukherjee
Publisher:
ISBN:
Category : Antiferromagnetism
Languages : en
Pages : 418

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Author: David Macdougal
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Category :
Languages : en
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Publisher: Elsevier
ISBN: 0128020938
Category : Science
Languages : en
Pages : 534

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Neutron Scattering - Magnetic and Quantum Phenomena provides detailed coverage of the application of neutron scattering in condensed matter research. The book's primary aim is to enable researchers in a particular area to identify the aspects of their work where neutron scattering techniques might contribute, conceive the important experiments to be done, assess what is required to carry them out, write a successful proposal for one of the major user facilities, and perform the experiments under the guidance of the appropriate instrument scientist. An earlier series edited by Kurt Sköld and David L. Price, and published in the 1980s by Academic Press as three volumes in the series Methods of Experimental Physics, was very successful and remained the standard reference in the field for several years. This present work has similar goals, taking into account the advances in experimental techniques over the past quarter-century, for example, neutron reflectivity and spin-echo spectroscopy, and techniques for probing the dynamics of complex materials of technological relevance. This volume complements Price and Fernandez-Alonso (Eds.), Neutron Scattering - Fundamentals published in November 2013. Covers the application of neutron scattering techniques in the study of quantum and magnetic phenomena, including superconductivity, multiferroics, and nanomagnetism Presents up-to-date reviews of recent results, aimed at enabling the reader to identify new opportunities and plan neutron scattering experiments in their own field Provides a good balance between theory and experimental techniques Provides a complement to Price and Fernandez-Alonso (Eds.), Neutron Scattering - Fundamentals published in November 2013

Author: Wei He (Researcher in materials science)
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Category :
Languages : en
Pages :

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The study of quantum magnets in two-dimensional systems is a forefront field in both materials science and condensed matter physics research. Such materials not only provide rich platforms for potential applications of novel materials but also further our understanding of basic physics. Neutron and x-ray scattering are powerful tools to explore the magnetic and charge correlations in these materials. This thesis describes the experimental investigation of two model systems in bulk crystalline form, one with a two-dimensional kagome lattice and one with a two-dimensional square lattice, both consisting of Cu2+ ions with spin-1/2. Strong quantum fluctuations give competing ground states or phases in both systems. Recently, barlowite Cu4(OH)6FBr has attracted much attention as the parent compound of a new kagome quantum spin liquid candidate. Our new synthesis method produced large single crystals of a new variant of barlowite, which has a higher symmetry space group compared to the previously reported one. Our elastic magnetic neutron scattering measurements reveal that the magnetic ground state of the new high-symmetry barlowite at low temperatures has a special pinwheel q = 0 magnetic order. In the intermediate temperatures, our numerical calculations and inelastic neutron scattering indicate that the kagome spins are in a potential pinwheel valence bond crystal state. Both of the two ground states are in close proximity to the long-sought quantum spin liquid state. The second part of my thesis is focused on the spin and charge correlations in high-Tc cuprate superconductors. Cuprate materials display intriguing physical phenomena due to the coexistence of various phases, which may interact with the superconductivity. The La-based family is a canonical example where both the spin and charge correlations could form "stripes". Magnetic neutron scattering reveals a rather surprising feature of the spin stripes in the model material La1.88Sr0.12CuO4: regardless of whether they are static or fluctuating, these stripes are always tilted from the high-symmetry direction of underlying lattices. Comparison with numerical simulations reveals the important role of the next-nearest neighbor electron hopping. Resonant soft x-ray scattering measurements offer important information about the charge order in another cuprate material stage-6 O-doped La2CuO4+y. By tuning both temperature and the dopant disorder level, we clearly observe two types of charge orders with distinct correlation lengths and behaviors at low temperatures. A coherent picture based on microscopic phase separation is proposed to explain the relationship between charge and spin orders with superconductivity in these materials.

Author: Michael Banton
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Category : Immigrants
Languages : en
Pages : 15

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Author: Miska Elliot
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Category :
Languages : en
Pages : 0

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Author: Ulrich Schollwöck
Publisher: Springer
ISBN: 3540400664
Category : Science
Languages : en
Pages : 488

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Closing a gap in the literature, this volume is intended both as an introductory text at postgraduate level and as a modern, comprehensive reference for researchers in the field. Provides a full working description of the main fundamental tools in the theorists toolbox which have proven themselves on the field of quantum magnetism in recent years. Concludes by focusing on the most important cuurent materials form an experimental viewpoint, thus linking back to the initial theoretical concepts.

Author: Viviane Peçanha Antonio
Publisher:
ISBN:
Category :
Languages : en
Pages : 0

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