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Author: Christoph Tobias Hebeisen Publisher: ISBN: 9780494590898 Category : Languages : en Pages : 220
Book Description
Ultrafast electron diffraction is a novel pump-probe technique which aims to determine transient structures during photoinduced chemical reactions and other structural transitions. This technique provides structural information at the atomic level of inspection by using an electron pulse as a diffractive probe. The atomic motions of interest happen on the 100 fs = 10-13 s time scale. To observe these atomic motions, a probe which matches this time scale is required. In this thesis, I describe the development of an electron diffractometer which is capable of 200 fs temporal resolution while maintaining high signal level per electron pulse. This was made possible by the construction of an ultra-compact photoactivated 60 keV femtosecond electron gun.Traditional electron pulse characterization methods are unsuitable for high number density femtosecond electron pulses such as the pulses produced by this electron gun. I developed two techniques based on the laser ponderomotive force to reliably determine the duration of femtosecond electron pulses into the sub-100 fs range. These techniques produce a direct cross-correlation trace between the electron pulse and a laser pulse. The results of these measurements confirmed the temporal resolution of the newly developed femtosecond electron diffractometer. This cross-correlation technique was also used to calibrate a method for the determination of the temporal overlap of electron and laser pulses. These techniques provide the pulse diagnostics necessary to utilize the temporal resolution provided by femtosecond electron pulses.Owing to their high charge-to-mass ratio, electrons are a sensitive probe for electric fields. I used femtosecond electron pulses in an electron deflectometry experiment to directly observe the transient charge distributions produced during femtosecond laser ablation of a silicon (100) surface. We found an electric field strength of 3.5 x 106 V/m produced by the emission of 5.3x1011 electrons/cm 2 just 3 ps after an excitation pulse of 5.6 J/cm2. This observation allowed us to rule out Coulomb explosion as the mechanism for ablation under the conditions present in this experiment.
Author: Christoph Tobias Hebeisen Publisher: ISBN: 9780494590898 Category : Languages : en Pages : 220
Book Description
Ultrafast electron diffraction is a novel pump-probe technique which aims to determine transient structures during photoinduced chemical reactions and other structural transitions. This technique provides structural information at the atomic level of inspection by using an electron pulse as a diffractive probe. The atomic motions of interest happen on the 100 fs = 10-13 s time scale. To observe these atomic motions, a probe which matches this time scale is required. In this thesis, I describe the development of an electron diffractometer which is capable of 200 fs temporal resolution while maintaining high signal level per electron pulse. This was made possible by the construction of an ultra-compact photoactivated 60 keV femtosecond electron gun.Traditional electron pulse characterization methods are unsuitable for high number density femtosecond electron pulses such as the pulses produced by this electron gun. I developed two techniques based on the laser ponderomotive force to reliably determine the duration of femtosecond electron pulses into the sub-100 fs range. These techniques produce a direct cross-correlation trace between the electron pulse and a laser pulse. The results of these measurements confirmed the temporal resolution of the newly developed femtosecond electron diffractometer. This cross-correlation technique was also used to calibrate a method for the determination of the temporal overlap of electron and laser pulses. These techniques provide the pulse diagnostics necessary to utilize the temporal resolution provided by femtosecond electron pulses.Owing to their high charge-to-mass ratio, electrons are a sensitive probe for electric fields. I used femtosecond electron pulses in an electron deflectometry experiment to directly observe the transient charge distributions produced during femtosecond laser ablation of a silicon (100) surface. We found an electric field strength of 3.5 x 106 V/m produced by the emission of 5.3x1011 electrons/cm 2 just 3 ps after an excitation pulse of 5.6 J/cm2. This observation allowed us to rule out Coulomb explosion as the mechanism for ablation under the conditions present in this experiment.
Author: Karsten König Publisher: Walter de Gruyter GmbH & Co KG ISBN: 3110383500 Category : Science Languages : en Pages : 360
Book Description
Nanostructuring of materials is a task at the heart of many modern disciplines in mechanical engineering, as well as optics, electronics, and the life sciences. This book includes an introduction to the relevant nonlinear optical processes associated with very short laser pulses for the generation of structures far below the classical optical diffraction limit of about 200 nanometers as well as coverage of state-of-the-art technical and biomedical applications. These applications include silicon and glass wafer processing, production of nanowires, laser transfection and cell reprogramming, optical cleaning, surface treatments of implants, nanowires, 3D nanoprinting, STED lithography, friction modification, and integrated optics. The book highlights also the use of modern femtosecond laser microscopes and nanoscopes as novel nanoprocessing tools.
Author: Markus Kitzler Publisher: Springer ISBN: 3319201735 Category : Science Languages : en Pages : 385
Book Description
This book documents the recent vivid developments in the research field of ultrashort intense light pulses for probing and controlling ultrafast dynamics. The recent fascinating results in studying and controlling ultrafast dynamics in ever more complicated systems such as (bio-)molecules and structures of meso- to macroscopic sizes on ever shorter time-scales are presented. The book is written by some of the most eminent experimental and theoretical experts in the field. It covers the new groundbreaking research directions that were opened by the availability of new light sources such as fully controlled intense laser fields with durations down to a single oscillation cycle, short-wavelength laser-driven attosecond pulses and intense X-ray pulses from the upcoming free electron lasers. These light sources allowed the investigation of dynamics in atoms, molecules, clusters, on surfaces and very recently also in nanostructures and solids in new regimes of parameters which, in turn, led to the identification of completely new dynamics and methods for controlling it. Example topics covered by this book include the study of ultrafast processes in large molecules using attosecond pulses, control of ultrafast electron dynamics in solids with shaped femtosecond laser pulses, light-driven ultrafast plasmonic processes on surfaces and in nanostructures as well as research on atomic and molecular systems under intense X-ray radiation. This book is equally helpful for people who would like to step into this field (e.g. young researchers), for whom it provides a broad introduction, as well as for already experienced researchers who may enjoy the exhaustive discussion that covers the research on essentially all currently studied objects and with all available ultrafast pulse sources.
Author: Franz X. Kärtner Publisher: Springer Science & Business Media ISBN: 9783540201151 Category : Science Languages : en Pages : 472
Book Description
This book covers the physics, technology and applications of short pulse laser sources that generate pulses with durations of only a few optical cycles. The basic design considerations for the different systems such as lasers, parametric amplifiers and external compression techniques which have emerged over the last decade are discussed to give researchers and graduate students a thorough introduction to this field. The existence of these sources has opened many new fields of research that were not possible before. These are UV and EUV generation from table-top systems using high-harmonic generation, frequency metrology enabling optical frequency counting, high-resolution optical coherence tomography, strong-field ultrafast solid-state processes and ultrafast spectroscopy, to mention only a few. Many new applications will follow. The book attempts to give a comprehensive, while not excessive, introduction to this exciting new field that serves both experienced researchers and graduate students entering the field. The first half of the book covers the current physical principles, processes and design guidelines to generate pulses in the optical range comprising only a few cycles of light. Such as the generation of relatively low energy pulses at high repetition rates directly from the laser, parametric generation of medium energy pulses and high-energy pulses at low repetition rates using external compression in hollow fibers. The applications cover the revolution in frequency metrology and high-resolution laser spectroscopy to electric field synthesis in the optical range as well as the emerging field of high-harmonic generation and attosecond science, high-resolution optical imaging and novel ultrafast dynamics in semiconductors. These fields benefit from the strong electric fields accompanying these pulses in solids and gases during events comprising only a few cycles of light.
Author: Claude Rulliere Publisher: Springer Science & Business Media ISBN: 0387266747 Category : Science Languages : en Pages : 438
Book Description
This smooth introduction for advanced undergraduates starts with the fundamentals of lasers and pulsed optics. Thus prepared, the student is introduced to short and ultrashort laser pulses, and learns how to generate, manipulate, and measure them. Spectroscopic implications are also discussed. The second edition has been completely revised and includes two new chapters on some of the most promising and fast-developing applications in ultrafast phenomena: coherent control and attosecond pulses.
Author: Jean-Claude Diels Publisher: Elsevier ISBN: 0080466400 Category : Science Languages : en Pages : 675
Book Description
Ultrashort Laser Pulse Phenomena, Second Edition serves as an introduction to the phenomena of ultra short laser pulses and describes how this technology can be used to examine problems in areas such as electromagnetism, optics, and quantum mechanics. Ultrashort Laser Pulse Phenomena combines theoretical backgrounds and experimental techniques and will serve as a manual on designing and constructing femtosecond ("faster than electronics") systems or experiments from scratch. Beyond the simple optical system, the various sources of ultrashort pulses are presented, again with emphasis on the basic concepts and how they apply to the design of particular sources (dye lasers, solid state lasers, semiconductor lasers, fiber lasers, and sources based on frequency conversion). - Provides an easy to follow guide through "faster than electronics" probing and detection methods - THE manual on designing and constructing femtosecond systems and experiments - Discusses essential technology for applications in micro-machining, femtochemistry, and medical imaging
Author: Richard Viskup Publisher: BoD – Books on Demand ISBN: 9535126067 Category : Science Languages : en Pages : 426
Book Description
This book gives the readers an introduction to experimental and theoretical knowledge acquired by large-scale laser laboratories that are dealing with extra-high peak power and ultrashort laser pulses for research of terawatt (TW), petawatt (PW), or near-future exawatt (EW) laser interactions, for soft X-ray sources, for acceleration of particles, or for generation of hot dense thermal plasma for the laser fusion. The other part of this book is dealing with the small-scale laser laboratories that are using for its research on commercial sources of laser radiation, nanosecond (ns), picosecond (ps), or femtosecond (fs) laser pulses, either for basic research or for more advanced applications. This book is divided into six main sections dealing with short and ultrashort laser pulses, laser-produced soft X-ray sources, large-scale high-power laser systems, free-electron lasers, fiber-based sources of short optical pulse, and applications of short pulse lasers. In each chapter readers can find fascinating topics related to the high energy and/or short pulse laser technique. Individual chapters should serve the broad spectrum of readers of different expertise, layman, undergraduate and postgraduate students, scientists, and engineers, who may in this book find easily explained fundamentals as well as advanced principles of particular subjects related to these phenomena.
Author: Jun Ye Publisher: Springer Science & Business Media ISBN: 0387237917 Category : Science Languages : en Pages : 373
Book Description
Over the last few years, there has been a convergence between the fields of ultrafast science, nonlinear optics, optical frequency metrology, and precision laser spectroscopy. These fields have been developing largely independently since the birth of the laser, reaching remarkable levels of performance. On the ultrafast frontier, pulses of only a few cycles long have been produced, while in optical spectroscopy, the precision and resolution have reached one part in Although these two achievements appear to be completely disconnected, advances in nonlinear optics provided the essential link between them. The resulting convergence has enabled unprecedented advances in the control of the electric field of the pulses produced by femtosecond mode-locked lasers. The corresponding spectrum consists of a comb of sharp spectral lines with well-defined frequencies. These new techniques and capabilities are generally known as “femtosecond comb technology. ” They have had dramatic impact on the diverse fields of precision measurement and extreme nonlinear optical physics. The historical background for these developments is provided in the Foreword by two of the pioneers of laser spectroscopy, John Hall and Theodor Hänsch. Indeed the developments described in this book were foreshadowed by Hänsch’s early work in the 1970s when he used picosecond pulses to demonstrate the connection between the time and frequency domains in laser spectroscopy. This work complemented the advances in precision laser stabilization developed by Hall.
Author: Susanne Yelin Publisher: Academic Press ISBN: 032398844X Category : Science Languages : en Pages : 148
Book Description
Advances in Atomic, Molecular, and Optical Physics, Volume 71 provides a comprehensive compilation of recent developments in a field that is in a state of rapid growth as new experimental and theoretical techniques are used on many problems, both old and new. Topics covered include related applied areas, such as atmospheric science, astrophysics, surface physics, and laser physics, with timely articles written by distinguished experts. Sample content covered in this release includes Attosecond generation and application from X-ray Free Electron Lasers. - Presents the work of international experts in the field - Contains comprehensive articles that compile recent developments in a field that is experiencing rapid growth, with new experimental and theoretical techniques emerging - Ideal for users interested in optics, excitons, plasmas and thermodynamics - Covers atmospheric science, astrophysics, and surface and laser physics, amongst other topics
Author: Publisher: Elsevier ISBN: 0128098945 Category : Science Languages : en Pages : 5276
Book Description
Encyclopedia of Interfacial Chemistry: Surface Science and Electrochemistry, Seven Volume Set summarizes current, fundamental knowledge of interfacial chemistry, bringing readers the latest developments in the field. As the chemical and physical properties and processes at solid and liquid interfaces are the scientific basis of so many technologies which enhance our lives and create new opportunities, its important to highlight how these technologies enable the design and optimization of functional materials for heterogeneous and electro-catalysts in food production, pollution control, energy conversion and storage, medical applications requiring biocompatibility, drug delivery, and more. This book provides an interdisciplinary view that lies at the intersection of these fields. Presents fundamental knowledge of interfacial chemistry, surface science and electrochemistry and provides cutting-edge research from academics and practitioners across various fields and global regions
Author: Christoph Tobias Hebeisen
Author: Christoph Tobias Hebeisen
Author: Karsten König
Author: Markus Kitzler
Author: Franz X. Kärtner
Author: Claude Rulliere
Author: Jean-Claude Diels
Author: Richard Viskup
Author: Jun Ye
Author: Susanne Yelin
Author: