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Femtosecond Filament Interaction as a Probe for Molecular Alignment

Femtosecond Filament Interaction as a Probe for Molecular Alignment PDF Author: Erik McKee
Publisher:
ISBN:
Category :
Languages : en
Pages : 82

Book Description
Femtosecond laser filamentation is a highly nonlinear propagation mode. When a laser pulse propagates with a peak power exceeding a critical value P[subscript cr] (5 GW at 800 nm in air), the Kerr effect tends to collapse the beam until the intensity is high enough to ionize the medium, giving rise to plasma defocusing. A dynamic competition between these two effects takes place leaving a thin and weakly ionized plasma channel in the trail of the pulse. When an ultrafast laser pulse interacts with molecules, it will align them, spinning them about their axis of polarization. As the quantum rotational wave packet relaxes, the molecules will experience periodic field-free alignment. Recent work has demonstrated the effect of molecular alignment on laser filamentation of ultra-short pulses. Revival of the molecular alignment can modify filamentation parameters as it can locally modify the refractive index and the ionization rate. In this thesis, we demonstrate with simulations and experiments that these changes in the filament parameters (collapse distance and filament plasma length) can be used to probe molecular alignment in CO2.

Femtosecond Filament Interaction as a Probe for Molecular Alignment

Femtosecond Filament Interaction as a Probe for Molecular Alignment PDF Author: Erik McKee
Publisher:
ISBN:
Category :
Languages : en
Pages : 82

Book Description
Femtosecond laser filamentation is a highly nonlinear propagation mode. When a laser pulse propagates with a peak power exceeding a critical value P[subscript cr] (5 GW at 800 nm in air), the Kerr effect tends to collapse the beam until the intensity is high enough to ionize the medium, giving rise to plasma defocusing. A dynamic competition between these two effects takes place leaving a thin and weakly ionized plasma channel in the trail of the pulse. When an ultrafast laser pulse interacts with molecules, it will align them, spinning them about their axis of polarization. As the quantum rotational wave packet relaxes, the molecules will experience periodic field-free alignment. Recent work has demonstrated the effect of molecular alignment on laser filamentation of ultra-short pulses. Revival of the molecular alignment can modify filamentation parameters as it can locally modify the refractive index and the ionization rate. In this thesis, we demonstrate with simulations and experiments that these changes in the filament parameters (collapse distance and filament plasma length) can be used to probe molecular alignment in CO2.

Progress in Ultrafast Intense Laser Science VIII

Progress in Ultrafast Intense Laser Science VIII PDF Author: Kaoru Yamanouchi
Publisher: Springer Science & Business Media
ISBN: 3642287263
Category : Science
Languages : en
Pages : 208

Book Description
The PUILS series delivers up-to-date reviews of progress in Ultrafast Intense Laser Science, a newly emerging interdisciplinary research field spanning atomic and molecular physics, molecular science and optical science which has been stimulated by the recent developments in ultrafast laser technologies. Each volume compiles peer-reviewed articles authored by researchers at the forefront of each their own subfields of UILS. Every chapter opens with an overview of the topics to be discussed, so that researchers unfamiliar to the subfield as well as graduate students can grasp the importance and attractions of the research topic at hand. These are followed by reports of cutting-edge discoveries. This eighth volume covers a broad range of topics from this interdisciplinary research field, focusing on molecules interacting with ultrashort and intense laser fields, advanced technologies for the characterization of ultrashort laser pulses and their applications, laser plasma formation and laser acceleration.

Femtosecond Laser Filamentation

Femtosecond Laser Filamentation PDF Author: See Leang Chin
Publisher: Springer Science & Business Media
ISBN: 1441906886
Category : Science
Languages : en
Pages : 138

Book Description
This book attempts to give a discussion of the physics and current and potential applications of the self-focusing of an intense femtosecond laser pulse in a tra- parent medium. Although self-focusing is an old subject of nonlinear optics, the consequence of self-focusing of intense femtosecond laser pulses is totally new and unexpected. Thus, new phenomena are observed, such as long range lam- tation, intensity clamping, white light laser pulse, self-spatial ltering, self-group phase locking, self-pulse compression, clean nonlinear uorescence, and so on. Long range propagation at high intensity, which is seemingly against the law of diffraction, is probably one of the most exciting consequences of this new sub- eld of nonlinear optics. Because the intensity inside the lament core is high, new ways of doing nonlinear optics inside the lament become possible. We call this lamentation nonlinear optics. We shall describe the generation of pulses at other wavelengths in the visible and ultraviolet (UV) starting from the near infrared pump pulse at 800 nm through four-wave-mixing and third harmonic generation, all in gases. Remotely sensing uorescence from the fragments of chemical and biological agents in all forms, gaseous, aerosol or solid, inside the laments in air is demonstrated in the labo- tory. The results will be shown in the last part of the book. Through analyzing the uorescence of gas molecules inside the lament, an unexpected physical process pertaining to the interaction of synchrotron radiation with molecules is observed.

Advances in Nonlinear Optics

Advances in Nonlinear Optics PDF Author: Xianfeng Chen
Publisher: Walter de Gruyter GmbH & Co KG
ISBN: 311030449X
Category : Science
Languages : en
Pages : 382

Book Description
This book presents an overview of the state of the art of the developing topic of nonlinear optics with contributions from leading experts in the field in China, ranging from weak light nonlinear optics, ultrafast nonlinear optics to electro-optical theory and applications. In the past decade, nonlinear optics has evolved into many different branches, depending on the form of the material used for studying the nonlinear phenomena. The growth of research in nonlinear optics is closely linked to the rapid technological advances that have occurred in related fields, such as ultra-fast phenomena and optical communications. Nonlinear-optics activities range from the fundamental studies of the interaction between matter and radiation to the development of devices, components, and systems of tremendous commercial interest for widespread applications in optical telecommunications, medicine, and biotechnology. This book reviews the development of some nonlinear optics researches in China, not only the discovery of new principles, but also potential applications of nonlinear optics for various industries.

Laser Physics

Laser Physics PDF Author:
Publisher:
ISBN:
Category : Lasers
Languages : en
Pages : 712

Book Description


Nonlinear Photonics and Novel Optical Phenomena

Nonlinear Photonics and Novel Optical Phenomena PDF Author: Zhigang Chen
Publisher: Springer
ISBN: 1461435382
Category : Science
Languages : en
Pages : 388

Book Description
Nonlinear Photonics and Novel Optical Phenomena contains contributed chapters from leading experts in nonlinear optics and photonics, and provides a comprehensive survey of fundamental concepts as well as hot topics in current research on nonlinear optical waves and related novel phenomena. The book covers self-accelerating airy beams, integrated photonics based on high index doped-silica glass, linear and nonlinear spatial beam dynamics in photonic lattices and waveguide arrays, the theory of polariton solitons in semiconductor microcavities, and Terahertz waves.

Optics Letters

Optics Letters PDF Author:
Publisher:
ISBN:
Category : Optics
Languages : en
Pages : 760

Book Description


Advances in Atomic, Molecular, and Optical Physics

Advances in Atomic, Molecular, and Optical Physics PDF Author:
Publisher: Academic Press
ISBN: 0123965373
Category : Science
Languages : en
Pages : 606

Book Description
Advances in Atomic, Molecular, and Optical Physics publishes reviews of recent developments in a field which is in a state of rapid growth, as new experimental and theoretical techniques are used on many old and new problems. Topics covered include related applied areas, such as atmospheric science, astrophysics, surface physics and laser physics. Articles are written by distinguished experts, and contain both relevant review material and detailed descriptions of important recent developments. - International experts - Comprehensive articles - New developments

Femtosecond Optical Frequency Comb: Principle, Operation and Applications

Femtosecond Optical Frequency Comb: Principle, Operation and Applications PDF Author: Jun Ye
Publisher: Springer Science & Business Media
ISBN: 0387237917
Category : Science
Languages : en
Pages : 373

Book Description
Over the last few years, there has been a convergence between the fields of ultrafast science, nonlinear optics, optical frequency metrology, and precision laser spectroscopy. These fields have been developing largely independently since the birth of the laser, reaching remarkable levels of performance. On the ultrafast frontier, pulses of only a few cycles long have been produced, while in optical spectroscopy, the precision and resolution have reached one part in Although these two achievements appear to be completely disconnected, advances in nonlinear optics provided the essential link between them. The resulting convergence has enabled unprecedented advances in the control of the electric field of the pulses produced by femtosecond mode-locked lasers. The corresponding spectrum consists of a comb of sharp spectral lines with well-defined frequencies. These new techniques and capabilities are generally known as “femtosecond comb technology. ” They have had dramatic impact on the diverse fields of precision measurement and extreme nonlinear optical physics. The historical background for these developments is provided in the Foreword by two of the pioneers of laser spectroscopy, John Hall and Theodor Hänsch. Indeed the developments described in this book were foreshadowed by Hänsch’s early work in the 1970s when he used picosecond pulses to demonstrate the connection between the time and frequency domains in laser spectroscopy. This work complemented the advances in precision laser stabilization developed by Hall.

Air Lasing

Air Lasing PDF Author: Pavel Polynkin
Publisher: Springer
ISBN: 3319652206
Category : Science
Languages : en
Pages : 152

Book Description
This book presents the first comprehensive, interdisciplinary review of the rapidly developing field of air lasing. In most applications of lasers, such as cutting and engraving, the laser source is brought to the point of service where the laser beam is needed to perform its function. However, in some important applications such as remote atmospheric sensing, placing the laser at a convenient location is not an option. Current sensing schemes rely on the detection of weak backscattering of ground-based, forward-propagating optical probes, and possess limited sensitivity. The concept of air lasing (or atmospheric lasing) relies on the idea that the constituents of the air itself can be used as an active laser medium, creating a backward-propagating, impulsive, laser-like radiation emanating from a remote location in the atmosphere. This book provides important insights into the current state of development of air lasing and its applications.