Electronic and nuclear quantum dynamics of molecules in intense laser fields PDF Download

Author: Yuichi Fujimura
Publisher: Frontiers Media SA
ISBN: 2832522114
Category : Science
Languages : en
Pages : 161

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Author: Dimitri Batani
Publisher: Springer Science & Business Media
ISBN: 1461513510
Category : Science
Languages : en
Pages : 409

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Book Description
The recent developement of high power lasers, delivering femtosecond pulses of 20 2 intensities up to 10 W/cm , has led to the discovery of new phenomena in laser interactions with matter. At these enormous laser intensities, atoms, and molecules are exposed to extreme conditions and new phenomena occur, such as the very rapid multi photon ionization of atomic systems, the emission by these systems of very high order harmonics of the exciting laser light, the Coulomb explosion of molecules, and the acceleration of electrons close to the velocity of light. These phenomena generate new behaviour of bulk matter in intense laser fields, with great potential for wide ranging applications which include the study of ultra-fast processes, the development of high-frequency lasers, and the investigation of the properties of plasmas and condensed matter under extreme conditions of temperature and pressure. In particular, the concept of the "fast ignitor" approach to inertial confinement fusion (ICF) has been proposed, which is based on the separation of the compression and the ignition phases in laser-driven ICF. The aim of this course on "Atom, Solids and Plasmas in Super-Intense Laser fields" was to bring together senior researchers and students in atomic and molecular physics, laser physics, condensed matter and plasma physics, in order to review recent developments in high-intensity laser-matter interactions. The course was held at the Ettore Majorana International Centre for Scientific Culture in Erice from July 8 to July 14,2000.

Author: Helene Lefebvre-Brion
Publisher: Elsevier
ISBN: 0080517501
Category : Science
Languages : en
Pages : 797

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Book Description
This book is written for graduate students just beginning research, for theorists curious about what experimentalists actually can and do measure, and for experimentalists bewildered by theory. It is a guide for potential users of spectroscopic data, and uses language and concepts that bridge the frequency-and time-domain spectroscopic communities. Key topics, concepts, and techniques include: the assignment of simple spectra, basic experimental techniques, definition of Born-Oppenheimer and angular momentum basis sets and the associated spectroscopic energy level patterns (Hund's cases), construction of effective Hamiltonian matrices to represent both spectra and dynamics, terms neglected in the Born-Oppenheimer approximation (situations intermediate between Hund's cases, spectroscopic perturbations), nonlinear least squares fitting, calculation and interpretation of coupling terms, semi-classical (WKB) approximation, transition intensities and interference effects, direct photofragmentation (dissociation and ionization) and indirect photofragmentation (predissociation and autoionization) processes, visualization of intramolecular dynamics, quantum beats and wavepackets, treatment of decaying quasi-eigenstates using a complex Heff model, and concluding with some examples of polyatomic molecule dynamics. Students will discover that there is a fascinating world of cause-and-effect localized dynamics concealed beyond the reduction of spectra to archival molecular constants and the exact ab initio computation of molecular properties. Professional spectroscopists, kinetics, ab initio theorists will appreciate the practical, simplified-model, and rigorous theoretical approaches discussed in this book. - A fundamental reference for all spectra of small, gas-phase molecules - It is the most up-to-date and comprehensive book on the electronic spectroscopy and dynamics of diatomic molecules - The authors pioneered the development of many of the experimental methods, concepts, models, and computational schemes described in this book

Author: Thomas Brabec
Publisher: Springer Science & Business Media
ISBN: 038740077X
Category : Technology & Engineering
Languages : en
Pages : 590

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Book Description
Due to the rapid progress in laser technology a wealth of novel fundamental and applied applications of lasers in atomic and plasma physics have become possible. This book focuses on the interaction of high intensity lasers with matter. It reviews the state of the art of high power laser sources, intensity laser-atom and laser-plasma interactions, laser matter interaction at relativistic intensities, and QED with intense lasers.

Author: Malte Oppermann
Publisher: Springer Science & Business Media
ISBN: 3319053388
Category : Science
Languages : en
Pages : 218

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This thesis presents an experimental study of the ultrafast molecular dynamics of CO_2^+ that are induced by a strong, near-infrared, femtosecond laser pulse. In particular, typical strong field phenomena such as tunneling ionisation, nonsequential double ionisation and photo-induced dissociation are investigated and controlled by employing an experimental technique called impulsive molecular alignment. Here, a first laser pulse fixes the molecule in space, such that the molecular dynamics can be studied as a function of the molecular geometry with a second laser pulse. The experiments are placed within the context of the study and control of ultrafast molecular dynamics, where sub-femtosecond (10^-15 seconds) resolution in ever larger molecular systems represents the current frontier of research. The thesis presents the required background in strong field and molecular physics, femtosecond laser architecture and experimental techniques in a clear and accessible language that does not require any previous knowledge in these fields.

Author: André D. Bandrauk
Publisher: CRC Press
ISBN: 9780824791759
Category : Science
Languages : en
Pages : 480

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Book Description
This text presents the major advances in both intense laser fields phenomena and laser control of photochemical reactions - highlighting experimental and theoretical research on the interaction of simple molecules with intense laser fields. The book introduces new concepts such as above-threshold ionization (ATI), above-threshold dissociation (ATD), laser-induced avoided crossings, and coherent control.

Author: Andre D Bandrauk
Publisher: Springer Science & Business Media
ISBN: 1461533643
Category : Science
Languages : en
Pages : 397

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Book Description
This volume contains the lectures and communications presented at the NATO Advanced Research Workshop (NATO ARW 900857) which was held May 5-10, 1991 at McMaster University, Hamilton, Ontario, Canada. A scientific commitee made up of P.P. Lambropoulos (USC & Crete), P.8. Corkum (NRC, Ottawa), and H. B. vL. van den Heuvell (FOM, Amsterdam) guided the organizers, A.D. Bandrauk (Sherbrooke) and S.C. Wallace (Toronto) in preparing a programme which would cover the latest advances in the field of atom and molecule laser interactions. Since the last meeting held in July 1987 on "Atomic and Molecular Processes with Short Intense Laser Pulses", NATO ASI vol 1718 (Plenum Press 1988), considerable progress has been made in understanding high intensity effects on atoms and the concomitant coherence effects. After four years, the emphasis is now shifting more to molecules. The present volume represents therefore this trend with four sections covering the main interests of research endeavours in this area: i) Atoms in Intense Laser-Fields ii) Molecules in Intense Laser Fields iii) Atomic Coherences iv) Molecular Coherences The experience developed over the years in multiphoton atomic processes has been very useful and is the main source of our understanding of similar processes in molecules. Thus ATI (above threshold ionization) has been found to occur in molecules as well as a new phenomenon, ATD (above-threshold dissociation). Laser-induced avoided crossings of molecular electronic surfaces is also now entering the current language of high intensity molecular processes.

Author: Kaoru Yamanouchi
Publisher: Springer
ISBN: 3319067311
Category : Science
Languages : en
Pages : 248

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Book Description
The PUILS series delivers up-to-date reviews of progress in Ultrafast Intense Laser Science, a newly emerging interdisciplinary research field spanning atomic and molecular physics, molecular science and optical science, which has been stimulated by the recent developments in ultrafast laser technologies. Each volume compiles peer-reviewed articles authored by researchers at the forefront of each their own subfields of UILS. Every chapter opens with an overview of the topics to be discussed, so that researchers unfamiliar to the subfield, as well as graduate students, can grasp the importance and attractions of the research topic at hand; these are followed by reports of cutting-edge discoveries. This eleventh volume covers a broad range of topics from this interdisciplinary research field, focusing on ultrafast dynamics of molecules in intense laser fields, pulse shaping techniques for controlling molecular processes, high-order harmonics generation and attosecond Photoionization, femtosecond laser induced filamentation and laser particle acceleration.

Author: A. L'Huillier
Publisher: Springer Science & Business Media
ISBN: 1461579635
Category : Science
Languages : en
Pages : 494

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Book Description
The rapid development of powerful pulsed lasers is at the origin of a conside rable interest in studying the response of an atom, a molecule (or a solid) to a strong electromagnetic field. It is now possible to produce at the laboratory scale, ultra-short 13 pulses with a duration of 100 femtoseconds (10- second) and a power of the order 12 of 1 terawatt (10 Watt). Under these conditions, very high peak intensities may be obtained and electric fields exceeding typical electron binding fields in atoms are generated. The interaction of an atom or a molecule with such electromagnetic fields has a highly non-linear character which leads to unexpected phenomena. Amongst them, - above-threshold ionization (ATI) i.e. the absorption of additional photons in excess of the minimal number necessary to overcome the ionization potential and its molecular counterpart, above-threshold dissociation (ATD); - generation of very high harmonics of the driving field; - stabilization of one-electron systems in strong fields. These processes were the main topics of two international meetings which were held in 1989 and 1991 in the United States under the common name SILAP (Super-Intense Laser-Atom Physics).

Author: H.G. Muller
Publisher: Springer Science & Business Media
ISBN: 9780792340485
Category : Science
Languages : en
Pages : 630

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Book Description
Atoms in strong radiation fields are interesting objects for study, and the research field that concerns itself with this study is a comparatively young one. For a long period after the ~scovery of the photoelectric effect. it was not possible to generate electro magnetic fields that did more than perturb the atom only slightly, and (first-or~er) perturbation theory could perfectly explain what was going on at those low intensities. The development of the pulsed laser bas changed this state of affairs in a rather dramatic way, and fields can be applied that really have a large, or even dominant influence on atomic structure. In the latter case, w~ speak of super-intense fields. Since the interaction between atoms and electromagnetic waves is characterized by many parameters other than the light intensity, such as frequency, iQnization potential, orbit time, etc., it is actually quite difficult to define what is exactly meant by the term 'super-intense'. Obviously the term does not have an absolute meaning, and intensity should always be viewed in relation to other properties of the system. An atom in a radiation field can thus best be described in terms of various ratios of the quantities involved. The nature of the system sometimes drastically changes if the value of one of these parameters exceeds a certain critical value, and the new regime could be called super-intense with respect to that parameter.