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Development and Application of Infrared and Tracer-based Planar Laser-induced Fluorescence Imaging Diagnostics

Development and Application of Infrared and Tracer-based Planar Laser-induced Fluorescence Imaging Diagnostics PDF Author: David A. Rothamer
Publisher:
ISBN: 9780549356424
Category :
Languages : en
Pages : 318

Book Description
IR-PLIF measurements of temperature and pressure are a new application of the technique. Initial IR-PLIF measurements focused on species concentrations of CO and CO2. The strong dependence of IR-PLIF signals on temperature and pressure indicated that IR-PLIF measurements of those quantities are possible.

Development and Application of Infrared and Tracer-based Planar Laser-induced Fluorescence Imaging Diagnostics

Development and Application of Infrared and Tracer-based Planar Laser-induced Fluorescence Imaging Diagnostics PDF Author: David A. Rothamer
Publisher:
ISBN: 9780549356424
Category :
Languages : en
Pages : 318

Book Description
IR-PLIF measurements of temperature and pressure are a new application of the technique. Initial IR-PLIF measurements focused on species concentrations of CO and CO2. The strong dependence of IR-PLIF signals on temperature and pressure indicated that IR-PLIF measurements of those quantities are possible.

Tracer-based Planar Laser-induced Fluorescence Diagnostics

Tracer-based Planar Laser-induced Fluorescence Diagnostics PDF Author: Brian Ho-yin Cheung
Publisher: Stanford University
ISBN:
Category :
Languages : en
Pages : 197

Book Description
Two advances to tracer-based planar laser-induced fluorescence (PLIF) diagnostics are presented in this work. The first improvement is the development of a 3-pentanone fluorescence quantum yield (FQY) database and model for a wide range of conditions in support of quantitative PLIF diagnostics. In addition, this work presents a sensitive, time-resolved tracer-based PLIF diagnostic, accomplished by using a continuous-wave (CW) laser with the high-FQY tracer toluene. Because of its ease of use and desirable photophysical properties, PLIF diagnostics using 3-pentanone as a tracer are common, particularly for internal combustion engine (ICE) diagnostics. Thus, there is a need for 3-pentanone FQY measurements and modeling over a wide range of temperatures, pressures, and excitation wavelengths. For insight into the collisionless process in the FQY model, measurements were made in 3-pentanone vapor at low-pressures across a range of temperatures using a flowing cell. Laser excitation with 248, 266, 277, 308 nm wavelengths were utilized, and Rayleigh scattering of the laser beam was used to calibrate the optical efficiency of the collection optics and detector. This low-pressure data allows calculation of the 3-pentanone fluorescence rate and non-radiative de-excitation rate in the fluorescence model. The vibrational relaxation cascade parameter for 3-pentanone collisions was also determined. Measurements of 3-pentanone FQY were also made over a range of temperatures and pressures relevant to diagnostic applications, and, in particular, combined high-temperature and high-pressure conditions applicable to internal combustion engines (ICE). These data were collected in a custom-built optical cell capable of simultaneous high-pressure and high-temperature conditions. The behavior of the FQY in nitrogen for temperatures up to 745 K and in air up to 570 K was examined for pressures from 1 to 25 bar. These data were used to further optimize the parameters in the FQY model representing collisional processes. The large quantity of data with 308 nm excitation allowed optimization of the nitrogen quenching rate, and data in air were used to optimize the oxygen quenching rate. These data were also used to optimize the vibrational relaxation parameters for nitrogen and oxygen. The model with the updated parameters is consistent with the data collected in the current work, as well as with fluorescence measurements made in optical ICEs up to 1100 K and 28 bar. Another area of tracer-based PLIF diagnostics development is time-resolved imaging. Because PLIF diagnostics are often performed using pulsed lasers, the time resolution of measurements is limited to the pulse rate of laser. Use of a high-powered visible laser with an off-the-shelf cavity frequency doubler is shown to produce a moderate-power CW beam in the ultraviolet wavelength regime. Application of this CW source to excite toluene, a high-FQY tracer, yields a sensitive, time-resolved tracer-based PLIF diagnostic. Fluctuation detection limits for tracer mole fraction were investigated by applying the diagnostic to an atmospheric temperature and pressure nitrogen jet seeded with 4% toluene, and detection limits of better than 1% of the maximum toluene mole fraction were achieved for detection of fluorescence signal at a point, along a line, and over a plane. The diagnostic was also demonstrated on a turbulent jet for line and planar detection and demonstrated the potential for toluene time-resolved PLIF diagnostics with CW lasers.

Tracer-based Planar Laser-induced Fluorescence Diagnostics

Tracer-based Planar Laser-induced Fluorescence Diagnostics PDF Author: Brian Ho-yin Cheung
Publisher:
ISBN:
Category :
Languages : en
Pages :

Book Description
Two advances to tracer-based planar laser-induced fluorescence (PLIF) diagnostics are presented in this work. The first improvement is the development of a 3-pentanone fluorescence quantum yield (FQY) database and model for a wide range of conditions in support of quantitative PLIF diagnostics. In addition, this work presents a sensitive, time-resolved tracer-based PLIF diagnostic, accomplished by using a continuous-wave (CW) laser with the high-FQY tracer toluene. Because of its ease of use and desirable photophysical properties, PLIF diagnostics using 3-pentanone as a tracer are common, particularly for internal combustion engine (ICE) diagnostics. Thus, there is a need for 3-pentanone FQY measurements and modeling over a wide range of temperatures, pressures, and excitation wavelengths. For insight into the collisionless process in the FQY model, measurements were made in 3-pentanone vapor at low-pressures across a range of temperatures using a flowing cell. Laser excitation with 248, 266, 277, 308 nm wavelengths were utilized, and Rayleigh scattering of the laser beam was used to calibrate the optical efficiency of the collection optics and detector. This low-pressure data allows calculation of the 3-pentanone fluorescence rate and non-radiative de-excitation rate in the fluorescence model. The vibrational relaxation cascade parameter for 3-pentanone collisions was also determined. Measurements of 3-pentanone FQY were also made over a range of temperatures and pressures relevant to diagnostic applications, and, in particular, combined high-temperature and high-pressure conditions applicable to internal combustion engines (ICE). These data were collected in a custom-built optical cell capable of simultaneous high-pressure and high-temperature conditions. The behavior of the FQY in nitrogen for temperatures up to 745 K and in air up to 570 K was examined for pressures from 1 to 25 bar. These data were used to further optimize the parameters in the FQY model representing collisional processes. The large quantity of data with 308 nm excitation allowed optimization of the nitrogen quenching rate, and data in air were used to optimize the oxygen quenching rate. These data were also used to optimize the vibrational relaxation parameters for nitrogen and oxygen. The model with the updated parameters is consistent with the data collected in the current work, as well as with fluorescence measurements made in optical ICEs up to 1100 K and 28 bar. Another area of tracer-based PLIF diagnostics development is time-resolved imaging. Because PLIF diagnostics are often performed using pulsed lasers, the time resolution of measurements is limited to the pulse rate of laser. Use of a high-powered visible laser with an off-the-shelf cavity frequency doubler is shown to produce a moderate-power CW beam in the ultraviolet wavelength regime. Application of this CW source to excite toluene, a high-FQY tracer, yields a sensitive, time-resolved tracer-based PLIF diagnostic. Fluctuation detection limits for tracer mole fraction were investigated by applying the diagnostic to an atmospheric temperature and pressure nitrogen jet seeded with 4% toluene, and detection limits of better than 1% of the maximum toluene mole fraction were achieved for detection of fluorescence signal at a point, along a line, and over a plane. The diagnostic was also demonstrated on a turbulent jet for line and planar detection and demonstrated the potential for toluene time-resolved PLIF diagnostics with CW lasers.

Strategies for Planar Laser-induced Fluorescence Thermometry in Shock Tube Flows

Strategies for Planar Laser-induced Fluorescence Thermometry in Shock Tube Flows PDF Author: Ji Hyung Yoo
Publisher: Stanford University
ISBN:
Category :
Languages : en
Pages : 151

Book Description
This thesis was motivated by the need to better understand the temperature distribution in shock tube flows, especially in the near-wall flow regions. Two main ideas in planar laser-induced fluorescence (PLIF) diagnostics are explored in this thesis. The first topic is the development of a single-shot PLIF diagnostic technique for quantitative temperature distribution measurement in shock tube flow fields. PLIF is a non-intrusive, laser-based diagnostic technique capable of instantaneously imaging key flow features, such as temperature, pressure, density, and species concentration, by measuring fluorescence signal intensity from laser-excited tracer species. This study performed a comprehensive comparison of florescence tracers and excitation wavelengths to determine the optimal combination for PLIF imaging in shock tube flow applications. Excitation of toluene at 248nm wavelength was determined to be the optimal strategy due to the resulting high temperature sensitivity and fluorescence signal level, compared to other ketone and aromatic tracers at other excitation wavelengths. Sub-atmospheric toluene fluorescence yield data was measured to augment the existing photophysical data necessary for this diagnostic technique. In addition, a new imaging test section was built to allow PLIF imaging in all regions of the shock tube test section, including immediately adjacent to the side and end walls. The signal-to-noise (SNR) and spatial resolution of the PLIF images were optimized using statistical analysis. Temperature field measurements were made with the PLIF diagnostic technique across normal incident and reflected shocks in the shock tube core flow. The resulting images show uniform spatial distribution, and good agreement with conditions calculated from the normal shock jump equations. Temperature measurement uncertainty is about 3.6% at 800K. The diagnostic was also applied to image flow over a wedge. The resulting images capture all the flow features predicted by numerical simulations. The second topic is the development of a quantitative near-wall diagnostic using tracer-based PLIF imaging. Side wall thermal boundary layers and end wall thermal layers are imaged to study the temperature distribution present under constant pressure conditions. The diagnostic technique validated in the shock tube core flow region was further optimized to improve near-wall image quality. The optimization process considered various wall materials, laser sheet orientations, camera collection angles, and optical components to find the configuration that provides the best images. The resulting images have increased resolution (15[Mu]m) and are able to resolve very thin non-uniform near-wall temperature layers (down to 60[Mu]m from the surface). The temperature field and thickness measurements of near-wall shock tube flows under various shock conditions and test gases showed good agreement with boundary layer theory. To conclude this thesis, new applications and future improvements to the developed PLIF diagnostic technique are discussed. These suggested refinements can provide an even more robust and versatile PLIF imaging technique capable of measuring a wider range of flow conditions near walls.

Applications of Planar Laser-induced Fluorescence Imaging Diagnostics to Reacting Flows

Applications of Planar Laser-induced Fluorescence Imaging Diagnostics to Reacting Flows PDF Author: P. H. Paul
Publisher:
ISBN:
Category :
Languages : en
Pages : 21

Book Description


Strategies for Planar Laser-induced Fluorescence Thermometry in Shock Tube Flows

Strategies for Planar Laser-induced Fluorescence Thermometry in Shock Tube Flows PDF Author: Ji Hyung Yoo
Publisher:
ISBN:
Category :
Languages : en
Pages :

Book Description
This thesis was motivated by the need to better understand the temperature distribution in shock tube flows, especially in the near-wall flow regions. Two main ideas in planar laser-induced fluorescence (PLIF) diagnostics are explored in this thesis. The first topic is the development of a single-shot PLIF diagnostic technique for quantitative temperature distribution measurement in shock tube flow fields. PLIF is a non-intrusive, laser-based diagnostic technique capable of instantaneously imaging key flow features, such as temperature, pressure, density, and species concentration, by measuring fluorescence signal intensity from laser-excited tracer species. This study performed a comprehensive comparison of florescence tracers and excitation wavelengths to determine the optimal combination for PLIF imaging in shock tube flow applications. Excitation of toluene at 248nm wavelength was determined to be the optimal strategy due to the resulting high temperature sensitivity and fluorescence signal level, compared to other ketone and aromatic tracers at other excitation wavelengths. Sub-atmospheric toluene fluorescence yield data was measured to augment the existing photophysical data necessary for this diagnostic technique. In addition, a new imaging test section was built to allow PLIF imaging in all regions of the shock tube test section, including immediately adjacent to the side and end walls. The signal-to-noise (SNR) and spatial resolution of the PLIF images were optimized using statistical analysis. Temperature field measurements were made with the PLIF diagnostic technique across normal incident and reflected shocks in the shock tube core flow. The resulting images show uniform spatial distribution, and good agreement with conditions calculated from the normal shock jump equations. Temperature measurement uncertainty is about 3.6% at 800K. The diagnostic was also applied to image flow over a wedge. The resulting images capture all the flow features predicted by numerical simulations. The second topic is the development of a quantitative near-wall diagnostic using tracer-based PLIF imaging. Side wall thermal boundary layers and end wall thermal layers are imaged to study the temperature distribution present under constant pressure conditions. The diagnostic technique validated in the shock tube core flow region was further optimized to improve near-wall image quality. The optimization process considered various wall materials, laser sheet orientations, camera collection angles, and optical components to find the configuration that provides the best images. The resulting images have increased resolution (15[Mu]m) and are able to resolve very thin non-uniform near-wall temperature layers (down to 60[Mu]m from the surface). The temperature field and thickness measurements of near-wall shock tube flows under various shock conditions and test gases showed good agreement with boundary layer theory. To conclude this thesis, new applications and future improvements to the developed PLIF diagnostic technique are discussed. These suggested refinements can provide an even more robust and versatile PLIF imaging technique capable of measuring a wider range of flow conditions near walls.

Advanced Diagnostics for Reacting Flows

Advanced Diagnostics for Reacting Flows PDF Author:
Publisher:
ISBN:
Category :
Languages : en
Pages : 17

Book Description
The goal of this research is to develop advanced laser-based techniques for non-intrusive measurements relevant to air-breathing combustion. In general, the program emphasizes spectrally-resolved absorption using tunable laser sources and planar laser-induced fluorescence (PLIF), conducted using either near-infrared or ultraviolet laser sources. Detailed below is progress on the exploration of IR PLIF as a diagnostic for imaging IR-active gases and on the suitability of pentanone as an alternative flow tracer to acetone for PLIF imaging. Furthermore, a novel absorption sensor for NO2 at temperatures up to 1900 K has been developed, and continuing work is reported on the spectroscopy of high-pressure gases.

Optical and Laser Diagnostics

Optical and Laser Diagnostics PDF Author: C Arcoumanis
Publisher: CRC Press
ISBN: 9780750309585
Category : Technology & Engineering
Languages : en
Pages : 274

Book Description
From the automotive industry to blood flow monitoring, optical techniques and laser diagnostics are becoming integral parts in engineering and medical instrumentation. Written by leading global experts from industry, academic groups, and laboratories, this volume provides an international perspective on both existing applications and leading-edge research. With a focus on advanced engineering applications, the book discusses the application of techniques such as laser Doppler velocimetry, particle image velocimetry, and planar laser-induced fluorescence to automotive engines, burners, and gas turbines. It also covers the flow, sprays, and combustion in direct-injection gasoline engines as well as the fundamental structure of flames as revealed by complementary laser techniques. In addition, the book explores laser diagnostic techniques used in the biomedical field and reviews novel research on the use of fiber-optic sensor techniques for structural integrity and physical condition monitoring.

Planar Laser-induced Fluorescence Imaging of Flame Heat Release Rate

Planar Laser-induced Fluorescence Imaging of Flame Heat Release Rate PDF Author:
Publisher:
ISBN:
Category :
Languages : en
Pages : 21

Book Description
Local heat release rate represents one of the most interesting experimental observables in the study of unsteady reacting flows. The direct measure of burning or heat release rate as a field variable is not possible. Numerous experimental investigations have relied on inferring this type of information as well as flame front topology from indirect measures which are presumed to be correlated. A recent study has brought into question many of the commonly used flame front marker and burning rate diagnostics. This same study found that the concentration of formyl radical offers the best possibility for measuring flame burning rate. However, primarily due to low concentrations, the fluorescence signal level from formyl is too weak to employ this diagnostic for single-pulse measurements of turbulent reacting flows. In this paper the authors describe and demonstrate a new fluorescence-based reaction front imaging diagnostic suitable for single-shot applications. The measurement is based on taking the pixel-by-pixel product of OH and CH2O planar laser-induced fluorescence images to yield an image closely related to a reaction rate. The spectroscopic and collisional processes affecting the measured signals are discussed and the foundation of the diagnostic, as based on laminar and unsteady flame calculations, is presented. The authors report the results of applying this diagnostic to the study of a laminar premixed flame subject to an interaction with an isolated line-vortex pair.

Industrial Applications of Laser Diagnostics

Industrial Applications of Laser Diagnostics PDF Author: Yoshihiro Deguchi
Publisher: Taylor & Francis
ISBN: 1439853398
Category : Science
Languages : en
Pages : 301

Book Description
Tighter regulations of harmful substances such as NOx, CO, heavy metals, particles, emissions from commercial plants and automobiles reflect a growing demand for lowering the anthropogenic burdens on the environment. It is equally important to monitor controlling factors to improve the operation of industrial machinery and plants. Among the many me