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All Optical Manipulation of a Single Nitrogen-vacancy Centre in Nanodiamond

All Optical Manipulation of a Single Nitrogen-vacancy Centre in Nanodiamond PDF Author: Michael Wolfgang Geiselmann
Publisher:
ISBN:
Category :
Languages : en
Pages : 123

Book Description
The efficient interaction of photons with single quantum emitters like nitrogen vacancy (NV) centres is essential for the elaboration of future integrated quantum optical devices. A promising strategy towards this goal capitalizes on the latest advances of nano-optics to boost the interaction with single emitters as well as strengthen coupling between several of them. However, fully exploiting the capabilities of this marriage between NV centres and optical nanostructures requires suitable tools to accurately control their interaction. In this thesis, we use optical manipulation to trap and manipulate in 3D individual nanodiamonds containing a single NV. We first demonstrate the use of optical tweezers as a tool to achieve deterministic trapping and three-dimensional spatial manipulation of individual nanodiamonds hosting a single NV spin. Remarkably, we find that the NV axis is nearly fixed inside the trap and can be controlled in situ by adjusting the polarization of the trapping light. By combining this unique spatial and angular control with coherent manipulation of the NV spin and fluorescence lifetime measurements near an integrated photonic system, we demonstrate individual optically trapped NV centers as a novel route for both three-dimensional vectorial magnetometry and sensing of the electromagnetic local density of states. In a second step, our manipulation technique is further developed to deterministically position a single nanodiamond into the hotspot of a plasmonic antenna. The gradient force of electromagnetic field of the excited plasmon acts as localized optical tweezers to drive the functionalized nanodiamonds to the regions of largest field enhancement of the antenna, where they are adsorbed. The proximity of the immobilized NV to the nano-antenna is corroborated by the observed decrease in its fluorescence lifetime. Last but not least, we observe a NV fluorescence decrease upon near-infrared (NIR) illumination. We identify the promotion of the excited electron to a so far unknown dark band with a fast decay channel as the origin of the fluorescence decrease. This assumption is verified by the excellent agreement between our simple rate equation model and the experiment. With this mechanism we demonstrate that a single NV can operate as an efficient and fast optical switch controlled through an independent NIR gating laser. Furthermore the hybrid system formed by a single NV coupled to a gold gap antenna enhances the modulation depth. The results presented in this thesis show the ability to manipulate and position NV centres in nanodiamond with optical tweezers. This paves the way towards spin based magnetic field and temperature sensing in liquid environment. Furthermore, the control of positioning and coupling to photonic and plasmonic nanostructures may play a role for potential applications in all-optical circuits or quantum optical devices.

All Optical Manipulation of a Single Nitrogen-vacancy Centre in Nanodiamond

All Optical Manipulation of a Single Nitrogen-vacancy Centre in Nanodiamond PDF Author: Michael Wolfgang Geiselmann
Publisher:
ISBN:
Category :
Languages : en
Pages : 123

Book Description
The efficient interaction of photons with single quantum emitters like nitrogen vacancy (NV) centres is essential for the elaboration of future integrated quantum optical devices. A promising strategy towards this goal capitalizes on the latest advances of nano-optics to boost the interaction with single emitters as well as strengthen coupling between several of them. However, fully exploiting the capabilities of this marriage between NV centres and optical nanostructures requires suitable tools to accurately control their interaction. In this thesis, we use optical manipulation to trap and manipulate in 3D individual nanodiamonds containing a single NV. We first demonstrate the use of optical tweezers as a tool to achieve deterministic trapping and three-dimensional spatial manipulation of individual nanodiamonds hosting a single NV spin. Remarkably, we find that the NV axis is nearly fixed inside the trap and can be controlled in situ by adjusting the polarization of the trapping light. By combining this unique spatial and angular control with coherent manipulation of the NV spin and fluorescence lifetime measurements near an integrated photonic system, we demonstrate individual optically trapped NV centers as a novel route for both three-dimensional vectorial magnetometry and sensing of the electromagnetic local density of states. In a second step, our manipulation technique is further developed to deterministically position a single nanodiamond into the hotspot of a plasmonic antenna. The gradient force of electromagnetic field of the excited plasmon acts as localized optical tweezers to drive the functionalized nanodiamonds to the regions of largest field enhancement of the antenna, where they are adsorbed. The proximity of the immobilized NV to the nano-antenna is corroborated by the observed decrease in its fluorescence lifetime. Last but not least, we observe a NV fluorescence decrease upon near-infrared (NIR) illumination. We identify the promotion of the excited electron to a so far unknown dark band with a fast decay channel as the origin of the fluorescence decrease. This assumption is verified by the excellent agreement between our simple rate equation model and the experiment. With this mechanism we demonstrate that a single NV can operate as an efficient and fast optical switch controlled through an independent NIR gating laser. Furthermore the hybrid system formed by a single NV coupled to a gold gap antenna enhances the modulation depth. The results presented in this thesis show the ability to manipulate and position NV centres in nanodiamond with optical tweezers. This paves the way towards spin based magnetic field and temperature sensing in liquid environment. Furthermore, the control of positioning and coupling to photonic and plasmonic nanostructures may play a role for potential applications in all-optical circuits or quantum optical devices.

Fluorescent Nanodiamonds

Fluorescent Nanodiamonds PDF Author: Huan-Cheng Chang
Publisher: John Wiley & Sons
ISBN: 1119477085
Category : Science
Languages : en
Pages : 294

Book Description
The most comprehensive reference on fluorescent nanodiamond physical and chemical properties and contemporary applications Fluorescent nanodiamonds (FNDs) have drawn a great deal of attention over the past several years, and their applications and development potential are proving to be manifold and vast. The first and only book of its kind, Fluorescent Nanodiamonds is a comprehensive guide to the basic science and technical information needed to fully understand the fundamentals of FNDs and their potential applications across an array of domains. In demonstrating the importance of FNDs in biological applications, the authors bring together all relevant chemistry, physics, materials science and biology. Nanodiamonds are produced by powerful cataclysmic events such as explosions, volcanic eruptions and meteorite impacts. They also can be created in the lab by high-pressure high-temperature treatment of graphite or detonating an explosive in a reactor vessel. A single imperfection can give a nanodiamond a specific, isolated color center which allows it to function as a single, trapped atom. Much smaller than the thickness of a human hair, a nanodiamond can have a huge surface area that allows it to bond with a variety of other materials. Because of their non-toxicity, nanodiamonds may be useful in biomedical applications, such as drug delivery and gene therapy. The most comprehensive reference on a topic of rapidly increasing interest among academic and industrial researchers across an array of fields Includes numerous case studies and practical examples from many areas of research and industrial applications, as well as fascinating and instructive historical perspectives Each chapter addresses, in-depth, a single integral topic including the fundamental properties, synthesis, mechanisms and functionalisation of FNDs The first book published by the key patent holder with his research group in the field of FNDs Fluorescent Nanodiamonds is an important working resource for a broad range of scientists and engineers in industry and academia. It will also be a welcome reference for instructors in chemistry, physics, materials science, biology and related fields.

Optical Magnetometry

Optical Magnetometry PDF Author: Dmitry Budker
Publisher: Cambridge University Press
ISBN: 1107010357
Category : Science
Languages : en
Pages : 431

Book Description
Comprehensive coverage of the principles, technology and diverse applications of optical magnetometry for graduate students and researchers in atomic physics.

Optical Properties of Diamond

Optical Properties of Diamond PDF Author: A.M. Zaitsev
Publisher: Springer Science & Business Media
ISBN: 3662045486
Category : Science
Languages : en
Pages : 508

Book Description
This handbook is the most comprehensive compilation of data on the optical properties of diamond ever written. It presents a multitude of data previously for the first time in English. The author provides quick access to the most comprehensive information on all aspects of the field.

Carbon Nanoparticles and Nanostructures

Carbon Nanoparticles and Nanostructures PDF Author: Nianjun Yang
Publisher: Springer
ISBN: 3319287826
Category : Technology & Engineering
Languages : en
Pages : 360

Book Description
This book focuses on carbon dots and diamonds, briefly covering other nanocarbon structures such as nanohorns and nanofibers. In the first part, chemical synthesis of carbon dots, their optical properties and their applications for sensing, catalytic reactions, bio-imaging and drug delivery are presented. The second part of the book deals with the preparation and purification of diamond nanoparticles, their properties and surface chemistry as well as the applications of diamond nanoparticles for seeding, bio-imaging and drug delivery. In the third and last part of the book, other nanostructures such as carbon nanofibers and carbon nanohorns are presented, including their application in electrochemistry, biochemistry and energy.

Photonic Applications and Hybrid Integration of Single Nitrogen Vacancy Centres in Nanodiamond

Photonic Applications and Hybrid Integration of Single Nitrogen Vacancy Centres in Nanodiamond PDF Author:
Publisher:
ISBN:
Category :
Languages : en
Pages : 225

Book Description


Coherent Control of a Single Nitrogen-vacancy Center Spin in an Optically Levitated Nanodiamond

Coherent Control of a Single Nitrogen-vacancy Center Spin in an Optically Levitated Nanodiamond PDF Author: Yi Zhang
Publisher:
ISBN:
Category :
Languages : en
Pages : 58

Book Description


The Properties of Nitrogen-vacancy Centres in Nanodiamond

The Properties of Nitrogen-vacancy Centres in Nanodiamond PDF Author: Carlo Bradac
Publisher:
ISBN:
Category : Diamonds
Languages : en
Pages : 233

Book Description
Diamond is unique. Whether mechanical, thermal, electrical or optical, its properties are within the most extreme compared to those of any other material. This, together with the fact that in the last fifty years the synthesis of artificial diamond has become a reality, makes it very attractive for engineering and technological purposes. The range of diamond-based applications is very diverse and, among the others, includes its use in mechanical machining, high-power high-frequency electronics and high transmissivity optics. -- Diamond is also host to a wide variety of crystallographic defects. Appropriately controlled, they can be used to tune the characteristics of the material, but even more interestingly they often possess attractive optical properties on their own. In particular, nitrogen-vacancy (NV) centres in diamond have been the subject of extensive study in the last few years. They possess unique room-temperature optical and spin properties which make them promising systems for solid-state qubits in quantum information technologies and for emerging applications in biotechnology, nanomedicine and high resolution magnetometry, such as drug delivery, fluorescent biomarking and spin imaging. -- This thesis is focused on NV centres in diamond. I first present an extensive review on diamond as a material, describing in detail its physical properties, the methods that have been developed to synthesise it and some of its possible applications. I then move the attention specifically to NV centres in nanodiamonds (NDs), i.e. diamond crystals in the nanometre size range (0-100 nm). They are a potential candidate for emerging technologies including high-resolution magnetometry and biomedical imaging. For these applications, specific material requirements, such as the small size of the diamond nanocrystals and the optical stability of the hosted NV centres, are crucial. The NV stability with respect to the nanodiamond size and surface is the central theme of this thesis. I analyse the optical behaviour of NV centres in nanodiamond while varying a number of key parameters such as size, surface termination and diamond origin. Based on the measurements, I conclude whether the nanodiamond size and the NV surface proximity are factors that must be taken into consideration in order to control the material and realise nanotechnologies based on NV centres in nanodiamonds.

High Sensitivity Magnetometers

High Sensitivity Magnetometers PDF Author: Asaf Grosz
Publisher: Springer
ISBN: 3319340700
Category : Technology & Engineering
Languages : en
Pages : 576

Book Description
This book gathers, for the first time, an overview of nearly all of the magnetic sensors that exist today. The book is offering the readers a thorough and comprehensive knowledge from basics to state-of-the-art and is therefore suitable for both beginners and experts. From the more common and popular AMR magnetometers and up to the recently developed NV center magnetometers, each chapter is describing a specific type of sensor and providing all the information that is necessary to understand the magnetometer behavior including theoretical background, noise model, materials, electronics, design and fabrication techniques, etc.

Quantum Information Processing with Diamond

Quantum Information Processing with Diamond PDF Author: Steven Prawer
Publisher: Elsevier
ISBN: 0857096680
Category : Science
Languages : en
Pages : 367

Book Description
Diamond nitrogen vacancy (NV) color centers can transform quantum information science into practical quantum information technology, including fast, safe computing. Quantum Information Processing with Diamond looks at the principles of quantum information science, diamond materials, and their applications. Part one provides an introduction to quantum information processing using diamond, as well as its principles and fabrication techniques. Part two outlines experimental demonstrations of quantum information processing using diamond, and the emerging applications of diamond for quantum information science. It contains chapters on quantum key distribution, quantum microscopy, the hybridization of quantum systems, and building quantum optical devices. Part three outlines promising directions and future trends in diamond technologies for quantum information processing and sensing. Quantum Information Processing with Diamond is a key reference for R&D managers in industrial sectors such as conventional electronics, communication engineering, computer science, biotechnology, quantum optics, quantum mechanics, quantum computing, quantum cryptology, and nanotechnology, as well as academics in physics, chemistry, biology, and engineering. - Brings together the topics of diamond and quantum information processing - Looks at applications such as quantum computing, neural circuits, and in vivo monitoring of processes at the molecular scale