Air-quality Modeling and Source-apportionment of Fine Particulate Matter: Implications and Applications in Time-series Health Studies PDF Download

Author: Amit Marmur
Publisher:
ISBN: 9781109871142
Category :
Languages : en
Pages : 186

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Book Description
Air-quality modeling tools may be useful in such investigations of the health effects of air-pollution and PM2.5 specifically. Emissions-based three-dimensional air quality models may introduce several benefits when applied in epidemiologic studies, such as improved spatial representativeness and availability/continuity of data, as well as information on source impacts. Receptor-based models are a common tool for apportioning of ambient levels of pollutants among the major contributing sources, and can be useful in discerning the relative health impacts of different sources.

Author: Sivaraman Balachandran
Publisher:
ISBN:
Category : Air
Languages : en
Pages :

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Book Description
Ambient and indoor air pollution is a major cause of premature mortality, and has been associated with more than three million preventative deaths per year worldwide. Most of these health impacts are from the effects from fine particulate matter. It is suspected that PM2.5 health effects vary by composition, which depends on the mixture of pollutants emitted by sources. This has led to efforts to estimate relationships between sources of PM2.5 and health effects. The health effects of PM2.5 may be preferentially dependent on specific species; however, recent work has suggested that health impacts may actually be caused by the net effect of the mixture of pollutants which make up PM2.5. Recently, there have been efforts to use source impacts from source apportionment (SA) studies as a proxy for these multipollutant effects. Source impacts can be quantified using both receptor and chemical transport models (RMs and CTMs), and have both advantages and limitations for their use in health studies. In this work, a technique is developed that reconciles differences between source apportionment (SA) models by ensemble-averaging source impacts results from several SA models. This method uses a two-step process to calculate the ensemble average. An initial ensemble average is used calculate new estimates of uncertainties for the individual SA methods that are used in the ensemble. Next, an updated ensemble average is calculated using the SA method uncertainties as weights. Finally, uncertainties of the ensemble average are calculated using propagation of errors that includes covariance terms. The ensemble technique is extended to include a Bayesian formulation of weights used in ensemble-averaging source impacts. In a Bayesian approach, probabilistic distributions of the parameters of interest are estimated using prior distributions, along with information from observed data. Ensemble averaging results in updated estimates of source impacts with lower uncertainties than individual SA methods. Overall uncertainties for ensemble-averaged source impacts were ~45 - 74%. The Bayesian approach also captures the expected seasonal variation of biomass burning and secondary impacts. Sensitivity analysis found that using non-informative prior weighting performed better than using weighting based on method-derived uncertainties. The Bayesian-based source impacts for biomass burning correlate better with observed levoglucosan (R2=0.66) and water soluble potassium (R2=0.63) than source impacts estimated using more traditional methods, and more closely agreed with observed total mass. Power spectra of the time series of biomass burning source impacts suggest that profiles/factors associated with this source have the greatest variability across methods and locations. A secondary focus of this work is to examine the impacts of biomass burning. First a field campaign was undertaken to measure emissions from prescribed fires. An emissions factor of 14±17 g PM2.5/kg fuel burned was determined. Water soluble organic carbon (WSOC) was highly correlated with potassium (K) (R2=.93) and levoglucosan (R2=0.98). Results using a biomass burning source profile derived from this work further indicate that source apportionment is sensitive to levels of potassium in biomass burning source profiles, underscoring the importance of quantifying local biomass burning source profiles. Second, the sensitivity of ambient PM2.5 to various fire and meteorological parameters in was examined using the method of principle components regression (PCR) to estimate sensitivity of PM2.5 to fire data and, observed and forecast meteorological parameters. PM2.5 showed significant sensitivity to PB, with a unit-based sensitivity of 3.2±1 æg m-3 PM2.5 per 1000 acres burned. PM2.5 had a negative sensitivity to dispersive parameters such as wind speed.

Author: Douw Steyn
Publisher: Springer
ISBN: 331904379X
Category : Science
Languages : en
Pages : 624

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Book Description
Recent developments in air pollution modelling are explored as a series of contributions from researchers at the forefront of their field. This newest contribution on air pollution modelling and its application is focused on local, urban, regional and intercontinental modelling; data assimilation and air quality forecasting; model assessment and evaluation; aerosol transformation. Additionally, this work also examines the relationship between air quality and human health and the effects of climate change on air quality. The work derives from a series of papers presented at the 33rd International Technical Meeting on Air Pollution Modelling and its Application held in Miami, USA, August 27 - 31, 2013. The book is intended as reference material for students and professors interested in air pollution modelling at the graduate level as well as researchers and professionals involved in developing and utilizing air pollution models.

Author: Barbara J. Finlayson-Pitts
Publisher: Elsevier
ISBN: 0080529070
Category : Science
Languages : en
Pages : 993

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Book Description
Here is the most comprehensive and up-to-date treatment of one of the hottest areas of chemical research. The treatment of fundamental kinetics and photochemistry will be highly useful to chemistry students and their instructors at the graduate level, as well as postdoctoral fellows entering this new, exciting, and well-funded field with a Ph.D. in a related discipline (e.g., analytical, organic, or physical chemistry, chemical physics, etc.). Chemistry of the Upper and Lower Atmosphere provides postgraduate researchers and teachers with a uniquely detailed, comprehensive, and authoritative resource. The text bridges the "gap" between the fundamental chemistry of the earth's atmosphere and "real world" examples of its application to the development of sound scientific risk assessments and associated risk management control strategies for both tropospheric and stratospheric pollutants. Serves as a graduate textbook and "must have" reference for all atmospheric scientists Provides more than 5000 references to the literature through the end of 1998 Presents tables of new actinic flux data for the troposphere and stratospher (0-40km) Summarizes kinetic and photochemical date for the troposphere and stratosphere Features problems at the end of most chapters to enhance the book's use in teaching Includes applications of the OZIPR box model with comprehensive chemistry for student use

Author: Lixin Li
Publisher: Elsevier
ISBN: 012816526X
Category : Computers
Languages : en
Pages : 336

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Book Description
Spatiotemporal Analysis of Air Pollution and Its Application in Public Health reviews, in detail, the tools needed to understand the spatial temporal distribution and trends of air pollution in the atmosphere, including how this information can be tied into the diverse amount of public health data available using accurate GIS techniques. By utilizing GIS to monitor, analyze and visualize air pollution problems, it has proven to not only be the most powerful, accurate and flexible way to understand the atmosphere, but also a great way to understand the impact air pollution has in diverse populations. This book is essential reading for novices and experts in atmospheric science, geography and any allied fields investigating air pollution. Introduces readers to the benefits and uses of geo-spatiotemporal analyses of big data to reveal new and greater understanding of the intersection of air pollution and health Ties in machine learning to improve speed and efficacy of data models Includes developing visualizations, historical data, and real-time air pollution in large geographic areas

Author: Committee on Research Priorities for Airborne Particulate Matter
Publisher: National Academies Press
ISBN: 0309591929
Category : Science
Languages : en
Pages : 212

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Book Description
New National Ambient Air Quality Standards for airborne particles smaller than 2.5 micrometers, called PM2.5, were issued by the U.S. Environmental Protection Agency (EPA) amidst scientific uncertainty and controversy. In response to a request from Congress, Research Priorities for Airborne Particulate Matter, the first of four books in a series, offers a conceptual framework for an integrated national program of particulate-matter research, identifies the 10 most critical research needs linked to key policy-related scientific uncertainties, and describes the recommended timing and estimated costs of such research. The committee concludes that EPA should devote more resources to investigating the relationships between fixed-site outdoor monitoring data and actual human breathing-zone exposures to ambient particulate matter and to identifying the most biologically important constituents and characteristics of particulate matter through toxicological studies. The recommended research activities are critical to determining actual exposures of human subpopulations most susceptible to harm from the most hazardous constituents of particulate matter. Future research will be an investment in public health and a means to ensure that resources spent on control technology and regulatory compliance will have a reasonable probability of success.

Author: United States. Congress. Senate. Committee on Environment and Public Works
Publisher:
ISBN:
Category : Air
Languages : en
Pages : 216

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Author: John H. Seinfeld
Publisher: John Wiley & Sons
ISBN: 1118591364
Category : Science
Languages : en
Pages : 1249

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Book Description
Thoroughly restructured and updated with new findings and new features The Second Edition of this internationally acclaimed text presents the latest developments in atmospheric science. It continues to be the premier text for both a rigorous and a complete treatment of the chemistry of the atmosphere, covering such pivotal topics as: * Chemistry of the stratosphere and troposphere * Formation, growth, dynamics, and properties of aerosols * Meteorology of air pollution * Transport, diffusion, and removal of species in the atmosphere * Formation and chemistry of clouds * Interaction of atmospheric chemistry and climate * Radiative and climatic effects of gases and particles * Formulation of mathematical chemical/transport models of the atmosphere All chapters develop results based on fundamental principles, enabling the reader to build a solid understanding of the science underlying atmospheric processes. Among the new material are three new chapters: Atmospheric Radiation and Photochemistry, General Circulation of the Atmosphere, and Global Cycles. In addition, the chapters Stratospheric Chemistry, Tropospheric Chemistry, and Organic Atmospheric Aerosols have been rewritten to reflect the latest findings. Readers familiar with the First Edition will discover a text with new structures and new features that greatly aid learning. Many examples are set off in the text to help readers work through the application of concepts. Advanced material has been moved to appendices. Finally, many new problems, coded by degree of difficulty, have been added. A solutions manual is available. Thoroughly updated and restructured, the Second Edition of Atmospheric Chemistry and Physics is an ideal textbook for upper-level undergraduate and graduate students, as well as a reference for researchers in environmental engineering, meteorology, chemistry, and the atmospheric sciences. Click here to Download the Solutions Manual for Academic Adopters: http://www.wiley.com/WileyCDA/Section/id-292291.html

Author: Sponsored by The Health Effects Institute
Publisher: National Academies Press
ISBN: 0309037263
Category : Science
Languages : en
Pages : 703

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Book Description
"The combination of scientific and institutional integrity represented by this book is unusual. It should be a model for future endeavors to help quantify environmental risk as a basis for good decisionmaking." â€"William D. Ruckelshaus, from the foreword. This volume, prepared under the auspices of the Health Effects Institute, an independent research organization created and funded jointly by the Environmental Protection Agency and the automobile industry, brings together experts on atmospheric exposure and on the biological effects of toxic substances to examine what is knownâ€"and not knownâ€"about the human health risks of automotive emissions.

Author:
Publisher:
ISBN:
Category : Air
Languages : en
Pages : 308

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